J. Mater. Sci. Technol. ›› 2021, Vol. 61: 33-45.DOI: 10.1016/j.jmst.2020.05.025
• Research Article • Previous Articles Next Articles
Dan Zhanga, Qi Hanc, Kun Yud, Xiaopeng Luc, Ying Liue, Ze Lua, Qiang Wanga,b,*()
Received:
2019-12-30
Revised:
2020-05-10
Accepted:
2020-05-11
Published:
2021-01-20
Online:
2021-01-20
Contact:
Qiang Wang
Dan Zhang, Qi Han, Kun Yu, Xiaopeng Lu, Ying Liu, Ze Lu, Qiang Wang. Antibacterial activities against Porphyromonas gingivalis and biological characteristics of copper-bearing PEO coatings on magnesium[J]. J. Mater. Sci. Technol., 2021, 61: 33-45.
Coatings | Mg | Si | O | Cu |
---|---|---|---|---|
PEO | 36.7 | 20.3 | 42.9 | n.a. |
PEO-3Cu | 30.4 | 17.9 | 48.7 | 2.9 |
PEO-5Cu | 29.7 | 17.5 | 47.8 | 4.9 |
PEO-7Cu | 26.8 | 19.0 | 47.1 | 7.1 |
Table 1 Elemental composition of the coatings (wt.%).
Coatings | Mg | Si | O | Cu |
---|---|---|---|---|
PEO | 36.7 | 20.3 | 42.9 | n.a. |
PEO-3Cu | 30.4 | 17.9 | 48.7 | 2.9 |
PEO-5Cu | 29.7 | 17.5 | 47.8 | 4.9 |
PEO-7Cu | 26.8 | 19.0 | 47.1 | 7.1 |
Fig. 2. Cross-section morphology and elemental mapping of the PEO coatings: (a) PEO coating without the addition of Cu; (b) PEO-3Cu; (c) PEO-5Cu; (d) PEO-7Cu.
Fig. 4. Bacteria suspensions after standard film-covered tests: (a-d) Bacteria suspensions of PEO after 0 h, 3 h, 6 h, and 9 h; (e-h) Bacteria suspensions of PEO-3Cu after 0 h, 3 h, 6 h, and 9 h; (i-l) Bacteria suspensions of PEO-5Cu after 0 h, 3 h, 6 h, and 9 h; (m-p) Bacteria suspensions of PEO-7Cu after 0 h, 3 h, 6 h, and 9 h.
Fig. 5. Antibacterial abilities of PEO coatings. (a) Antibacterial rate of the PEO coatings at different culture time point; (b) Results of liquid growth inhibition assay.
Fig. 6. (a) Optical density of MC3T3-E1 cells in extraction medium of experimental samples measured by CCK8 test (n = 14, * p < 0.05 ** p < 0.01); (b) Relative growth rate (RGR) and cytotoxicity level at different detection period.
Fig. 7. Apoptosis rates of MC3T3-E1 cells cocultured with the experimental samples for 24 h (a-d) and 72 h (e-h). Q1: dead cells ((Annexin V-FITC)-/PI+); Q2: late apoptosis cells ((Annexin V-FITC)+/PI+); Q3: live cells ((Annexin V-FITC)-/PI-); Q4: early apoptosis cells ((Annexin V-FITC)+/PI-).
Fig. 8. Adhesion of MC3T3-E1 cells on different samples. (a) Cytoskeleton staining of MC3T3-E1 cells cocultured with the experimental samples for 4 h and 24 h; (b) DAPI for nuclei (blue) and rhodamine-phalloidin for F-actin stress fibers (red) double stain for 4 h and 24 h.
Fig. 9. Results of immersion tests. (a) pH value of pure Mg and different PEO coatings in Hank’s solution at 37 °C for 7 days of immersion; (b) Cu ion concentration of different PEO coatings in Hank’s solution at 37 °C for 7 days of immersion; (c) Mg ion concentration of different PEO coatings in Hank’s solution at 37 °C for 7 days of immersion.
Fig. 10. XRD results of different PEO coatings. (a) Immersed in Hank’s solution at 37 °C for 3 days; (b) Immersed in Hank’s solution at 37 °C for 7 days.
[1] |
W. Zhang, L.L. Tan, D.R. Ni, J.X. Chen, Y.C. Zhao, L. Liu, C.J. Shuai, K. Yang, A. Atrens, M.C. Zhao, J. Mater. Sci. Technol. 35 (2019) 777-783.
DOI URL |
[2] |
L.Y. Li, L.Y. Cui, R.C. Zeng, S.Q. Li, X.B. Chen, Y.F. Zheng, M.B. Kannand, Acta Biomater. 79 (2018) 23-36.
DOI URL PMID |
[3] |
L.L. Tan, L. Yu, P. Wan, K. Yang, J. Mater. Sci. Technol. 29 (2013) 503-513.
DOI URL |
[4] |
D.A. Robinson, R.W. Griffith, D. Shechtman, R.B. Evans, M.G. Conzemius, Acta Biomater. 6 (2010) 1869-1877.
DOI URL PMID |
[5] |
L. Ren, X. Lin, L.L. Tan, K. Yang, Mater. Lett. 65 (2011) 3509-3511.
DOI URL |
[6] |
R. Radha, D. Sreekanth, J. Magn. Alloys 5 (2017) 286-312.
DOI URL |
[7] |
Y. Shao, R.C. Zeng, A.Q. Li, L.Y. Cui, Y.H. Zou, S.K. Guan, Y.F. Zheng, Acta Metall. Sin. (Engl. Lett.) 33 (2020) 615-629.
DOI URL |
[8] | H.F. Li, Y.F. Zheng, L. Qin, Prog. Nat. Sci.: Mater.Int. 24 (2014) 414-422. |
[9] | F. Witte, Acta Biomater. 23 (2015) 528-540. |
[10] |
L.Y. Cui, G.B. Wei, R.C. Zeng, S.Q. Li, Y.H. Zou, E.H. Han, Bioact. Mater. 3 (2018) 245-249.
DOI URL PMID |
[11] | C.Y. Li, X.L. Fan, R.C. Zeng, L.Y. Cui, S.Q. Li, F. Zhang, Q.K. He, M.B. Kannan, H.W. (George) Jiang, D.C. Chen, S.K. Guan, J. Mater. Sci. Technol. 35 (2019) 1088-1098. |
[12] |
H.Q. Feng, G.M. Wang, W.H. Jin, X.M. Zhang, Y.F. Huang, A. Gao, H. Wu, G.S. Wu, P.K. Chu, ACS Appl. Mater. Interfaces 8 (2016) 9662-9673.
DOI URL PMID |
[13] |
M.I. Rahim, M. Rohde, B. Rais, J.M. Seitz, P.P. Mueller, J. Biomed. Mater. Res. A. 104 (2016) 1489-1499.
DOI URL PMID |
[14] |
P. Hou, C.L. Zhao, P.F. Cheng, H.L. Wu, J.H. Ni, S.X. Zhang, T.F. Lou, C.Y. Wang, X.N. Zhang Han, Y.M. Chai, Biomed. Mater. 12 (2016) 015010.
DOI URL PMID |
[15] |
C. Davide, M. Lucio, A.C. Renata, Biomaterials 34 (2013) 8018-8029.
URL PMID |
[16] | L.J. Heitz-Mayfield, J. Cliniic. Periodontol. 35 (2008) 292-304. |
[17] |
K. Sakai, T. Shibui, K. Sato, K. Hashimoto, T. Ushioda, N. Seta, S. Takahashi, T. Nomura, J. Oral Maxillofac. Surg. Med. Pathol. 30 (2018) 452-456.
DOI URL |
[18] |
R. Liu, K. Memarzadeh, B. Chang, Y.M. Zhang, Z. Ma, R.P. Allaker, L. Ren, K. Yang, Sci. Rep. 6 (2016) 29985.
URL PMID |
[19] | D. Lindsay, S. Holy, Can. J. Infect. Control 64 (2006) 313-325. |
[20] |
D. Zhang, L. Ren, Y. Zhang, N. Xue, K. Yang, M. Zhong, Colloids Surf. B Biointerfaces 105 (2013) 51-57.
URL PMID |
[21] |
L.Y. Cui, G.B. Wei, Z.Z. Han, R.C. Zeng, L. Wang, Y.H. Zou, S.Q. Li, D.K. Xu, S.K. Guan, J. Mater. Sci. Technol. 35 (2019) 254-265.
DOI URL |
[22] |
Y.B. Zhao, L.Q. Shi, X.J. Ji, Z.Z. Han, S.Q. Li, R.C. Zeng, F. Zhang, Z.L. Wang, J. Colloid Interface Sci. 526 (2018) 43-50.
DOI URL PMID |
[23] |
E. Dayaghi, H.R. Bakhsheshi-Rad, E. Hamzah, A. Akhavan-Farid, A.F. Ismail, M. Aziz, E. Abdolahi, Mater. Sci. Eng. C 102 (2019) 53-65.
DOI URL |
[24] |
X.J. Ji, L. Gao, J.C. Liu, J. Wang, Q. Cheng, J.P. Li, S.Q. Li, K.Q. Zhi, R.C. Zeng, Z.L. Wang, Colloids Surf. B Biointerfaces 179 (2019) 429-436.
URL PMID |
[25] |
Y.B. Zhao, X.Y. Chen, S.Q. Li, R.C. Zeng, F. Zhang, Z.L. Wang, S.K. Guan, J. Colloid Interface Sci. 547 (2019) 309-317.
DOI URL PMID |
[26] |
Y.B. Zhao, L.Q. Shi, X.J. Ji, Z.Z. Han, S.Q. Li, R.C. Zeng, F. Zhang, Z.L. Wang, J. Colloid Interface Sci. 526 (2018) 43-50.
URL PMID |
[27] |
Y. Li, L. Liu, P. Wan, Z.J. Zhai, Z.Y. Mao, Z.X. Ouyang, D.G. Yu, Q. Sun, L.L. Tan, L. Ren, Z.N. Zhu, Y.Q. Hao, X.H. Qu, K. Yang, K.R. Dai, Biomaterials 106 (2016) 250-263.
DOI URL PMID |
[28] |
S. Jin, D. Zhang, X.P. Lu, Y. Zhang, L.L. Tan, Y. Liu, Q. Wang, J. Mater. Sci. Technol. 47 (2020) 190-201.
DOI URL |
[29] |
X.D. Yan, P. Wan, L.L. Tan, M.C. Zhao, L. Qin, K. Yang, Mater. Sci. Eng. C 93 (2018) 565-581.
DOI URL |
[30] |
L. Ren, K. Yang, L. Guo, H.W. Chai, Mater. Sci. Eng. C 32 (2012) 1204-1209.
DOI URL |
[31] |
S. Wang, C. Yang, L. Ren, M.G. Shen, K. Yang, Mater. Lett. 129 (2014) 88-90.
DOI URL |
[32] |
T. Koyanagi, M. Sakamoto, Y. Takeuchi, M. Ohkuma, Y. Izumi, J. Oral Microbiology 2 (2010) 5104.
DOI URL |
[33] |
M. Vincent, R.E. Duval, P. Hartemann, M. Engels-Deutsch, J. Appl. Microbiol. 124 (2018) 1032-1046.
DOI URL PMID |
[34] |
J. Rosenbaum, D.L. Versace, S. Abbad-Andallousi, R. Pires, C. Azevedo, P. Cenedese, P. Dubot, Biomater. Sci. 5 (2017) 455-462.
DOI URL PMID |
[35] |
Z.L. Ding, Y. Wang, Q. Zhou, Z.Y. Ding, J. Liu, Q.G. He, H.B. Zhang, Biomolecules 10 (2020) 68.
DOI URL |
[36] |
J.Q. Song, P.L. Jin, M.Q. Li, J.G. Liu, D.M. Wu, H.T. Yao, J.Q. Wang, J. Mater. Sci. Mater. Med. 30 (2019) 49.
URL PMID |
[37] |
Y. Li, G.W. Liu, Z.J. Zhai, L.N. Liu, H.W. Li, K. Yang, L.L. Tan, P. Wan, X.Q. Liu, Z.X. Ouyang, Z.F. Yu, T.T. Tang, Z.N. Zhu, X.H. Qu, K.R. Dai, Antimicrob. Agents Chemother. 58 (2014) 7586-7591.
DOI URL PMID |
[38] |
A. Atrens, G.L. Song, F.Y. Cao, Z.M. Shi, P.K. Bowen, J. Magn. Alloys 1 (2013) 177-200.
DOI URL |
[39] |
A. Atrens, G.L. Song, M. Liu, Z.M. Shi, F.Y. Cao, M.S. Dargusch, Adv. Eng. Mater. 17 (2015) 400-453.
DOI URL |
[40] |
J.P. Lu, X. He, H.X. Li, R.G. Song, Materials 11 (2018) 1062.
DOI URL |
[41] |
X.P. Lu, C. Blawert, D. Tolnai, T. Subroto, K.U. Kainer, T. Zhang, F.H. Wang, M.L. Zheludkevich, Corros. Sci. 139 (2018) 395-402.
DOI URL |
[42] |
X.P. Lu, C. Blawert, Y.D. Huang, H. Ovri, M.L. Zheludkevich, K.U. Kainer, Electrochim. Acta 187 (2016) 20-33.
DOI URL |
[43] |
X.P. Lu, M. Mohedano, C. Blawert, E. Matykina, R. Arrabal, K.U. Kainer, M.L. Zheludkevich, Surf. Coat. Technol. 307 (2016) 1165-1182.
DOI URL |
[44] | L.F. Zhuang, R.M. Watt, N. Mattheos, M.S. Si, H.C. Lai, N.P. Lang, Clin. Oral Impl. Res. 27 (2016) 13-21. |
[45] |
A.J. Van Winkelhoff, R.J. Goené, C. Benschop, T. Flomer, Clin. Oral Impl. Res. 11 (2000) 511-520.
DOI URL |
[46] |
J.V. Rau, M. Curcio, M.G. Raucci, K. Barbaro, I. Fasolino, R. Teghil, L. Ambrosio, A.D. Bonis, A.R. Boccaccini, ACS Appl. Mater. Interfaces 11 (2019) 5812-5820.
URL PMID |
[47] |
L.L. Tan, Q. Wang, X. Lin, P. Wan, G.D. Zhang, Q. Zhang, K. Yang, Acta Biomater. 10 (2014) 2333-2340.
DOI URL PMID |
[48] |
M. Hans, S. Mathwes, F. Mucklich, M. Solioz, Biointerphases 11 (2016) 018902.
DOI URL PMID |
[49] |
J.X. Chen, W. Peng, L. Zhu, L.L. Tan, I.P. Etim, X.J. Wang, K. Yang, Mater. Technol. 33 (2018) 145-152.
DOI URL |
[50] |
F.I. Bussiere, E. Gueux, E. Rock, J.P. Girardeau, A. Tridon, A. Mazur, Y. Rayssiguier, Br. J. Nutr. 87 (2002) 107-113.
DOI URL PMID |
[51] |
M. Vincent, P. Harteman, M. Engels-Deutsch, Int. J. Hyg. Environ. Health 219 (2016) 585-591.
URL PMID |
[52] |
J.V. Rau, M. Curcio, M.G. Raucci, K. Barbaro, I. Fasolino, R. Teghil, L. Ambrosio, A.D. Bonis, A.R. Boccaccini, ACS Appl. Mater. Interfaces 11 (2019) 5812-5820.
DOI URL PMID |
[53] |
C. Liu, X.K. Fu, H.B. Pan, P. Wan, L. Wang, L.L. Tan, K.H. Wang, Y. Zhao, K. Yang, P.K. Chu, Sci. Rep. 6 (2016) 27374.
URL PMID |
[54] |
S. Galli, Y. Naito, J. Karlsson, W.X. He, I. Miyamoto, Y. Xue, M. Andersson, K. Mustafa, A. Wennerberg, R. Jimbo, Acta Biomater. 10 (2014) 5193-5201.
DOI URL PMID |
[55] |
D. Mushahary, C. Wen, J.M. Kunar, R. Sravanthi, P. Hodgson, G. Pande, Y.C. Li, Clin. Oral Implants Res. 27 (2016) E15-E24.
URL PMID |
[56] |
Y.Y. Yang, K. Zheng, R.F. Liang, A. Mainka, N. Taccardi, J.A. Roether, R. Detsch, W.H. Goldmann, S. Virtanen, A.R. Boccaccini, Biomed. Mater. 13 (2017) 015001.
URL PMID |
[57] |
L.Y. Cui, R.C. Zeng, S.K. Guan, W.C. Qi, F. Zhang, S.Q. Li, E.H. Han, J. Alloys. Compd. 695 (2017) 2464-2476.
DOI URL |
[58] |
J.X. Chen, Y. Zhang, M. Ibrahima, I.P. Etim, L.L. Tan, K. Yang, Colloids Surf. B Biointerfaces 179 (2019) 77-86.
DOI URL PMID |
[1] | Wei Feng, Nian Liu, Lingling Gao, Qian Zhou, Luofeng Yu, Xiaoting Ye, Jingjing Huo, Xiao Huang, Peng Li, Wei Huang. Rapid inactivation of multidrug-resistant bacteria and enhancement of osteoinduction via titania nanotubes grafted with polyguanidines [J]. J. Mater. Sci. Technol., 2021, 69(0): 188-199. |
[2] | Yuan Yu, Nannan Xu, Shengyu Zhu, Zhuhui Qiao, Jianbin Zhang, Jun Yang, Weimin Liu. A novel Cu-doped high entropy alloy with excellent comprehensive performances for marine application [J]. J. Mater. Sci. Technol., 2021, 69(0): 48-59. |
[3] | Shuai-Feng Chen, Hong-Wu Song, Ming Cheng, Ce Zheng, Shi-Hong Zhang, Myoung-Gyu Lee. Texture modification and mechanical properties of AZ31 magnesium alloy sheet subjected to equal channel angular bending [J]. J. Mater. Sci. Technol., 2021, 67(0): 211-225. |
[4] | Lingling Liu, Yeqiang Bu, Yue Sun, Jianfeng Pan, Jiabin Liu, Jien Ma, Lin Qiu, Youtong Fang. Trace bis-(3-sulfopropyl)-disulfide enhanced electrodeposited copper foils [J]. J. Mater. Sci. Technol., 2021, 74(0): 237-245. |
[5] | Longqing Tang, Guowei Bo, Fulin Jiang, Shiwei Xu, Jie Teng, Dingfa Fu, Hui Zhang. Unravelling the precipitation evolutions of AZ80 magnesium alloy during non-isothermal and isothermal processes [J]. J. Mater. Sci. Technol., 2021, 75(0): 184-195. |
[6] | Xu Han, Jianhua Wu, Xianhui Zhang, Junyou Shi, Jiaxin Wei, Yang Yang, Bo Wu, Yonghui Feng. Special issue on advanced corrosion-resistance materials and emerging applications. The progress on antifouling organic coating: From biocide to biomimetic surface [J]. J. Mater. Sci. Technol., 2021, 61(0): 46-62. |
[7] | Qianqian Jin, Xiaohong Shao, Shijian Zheng, Yangtao Zhou, Bo Zhang, Xiuliang Ma. Interfacial dislocations dominated lateral growth of long-period stacking ordered phase in Mg alloys [J]. J. Mater. Sci. Technol., 2021, 61(0): 114-118. |
[8] | Xian-Zong Wang, Hong-Qiang Fan, Triratna Muneshwar, Ken Cadien, Jing-Li Luo. Balancing the corrosion resistance and through-plane electrical conductivity of Cr coating via oxygen plasma treatment [J]. J. Mater. Sci. Technol., 2021, 61(0): 75-84. |
[9] | Zhihua Yu, Huimei Zhang, Jianying Huang, Shuhui Li, Songnan Zhang, Yan Cheng, Jiajun Mao, Xiuli Dong, Shouwei Gao, Shanchi Wang, Zhong Chen, Yaoxing Jiang, Yuekun Lai. Namib desert beetle inspired special patterned fabric with programmable and gradient wettability for efficient fog harvesting [J]. J. Mater. Sci. Technol., 2021, 61(0): 85-92. |
[10] | Huajing Xiong, Jianan Fu, Jinyao Li, Rashad Ali, Hong Wang, Yifan Liu, Hua Su, Yuanxun Li, Woon-Ming Lau, Nasir Mahmood, Chunhong Mu, Xian Jian. Strain-regulated sensing properties of α-Fe2O3 nano-cylinders with atomic carbon layers for ethanol detection [J]. J. Mater. Sci. Technol., 2021, 68(0): 132-139. |
[11] | Zhi-Jia Zhang, Wei-Jie Li, Shu-Lei Chou, Chao Han, Hua-Kun Liu, Shi-Xue Dou. Effects of carbon on electrochemical performance of red phosphorus (P) and carbon composite as anode for sodium ion batteries [J]. J. Mater. Sci. Technol., 2021, 68(0): 140-146. |
[12] | Mingjun Li, Christoph Schlaich, Jianguang Zhang, Ievgen S. Donskyi, Karin Schwibbert, Frank Schreiber, Yi Xia, Jörg Radnik, Tanja Schwerdtle, Rainer Haag. Mussel-inspired multifunctional coating for bacterial infection prevention and osteogenic induction [J]. J. Mater. Sci. Technol., 2021, 68(0): 160-171. |
[13] | J.X. Hou, X.Y. Li, K. Lu. Orientation dependence of mechanically induced grain boundary migration in nano-grained copper [J]. J. Mater. Sci. Technol., 2021, 68(0): 30-34. |
[14] | Xiaofan Zhai, Peng Ju, Fang Guan, Jizhou Duan, Nan Wang, Yimeng Zhang, Ke Li, Baorong Hou. Biofilm inhibition mechanism of BiVO4 inserted zinc matrix in marine isolated bacteria [J]. J. Mater. Sci. Technol., 2021, 75(0): 86-95. |
[15] | Qiyu Liao, Yanchao Jiang, Qichi Le, Xingrui Chen, Chunlong Cheng, Ke Hu, Dandan Li. Hot deformation behavior and processing map development of AZ110 alloy with and without addition of La-rich Mish Metal [J]. J. Mater. Sci. Technol., 2021, 61(0): 1-15. |
Viewed | ||||||
Full text |
|
|||||
Abstract |
|
|||||