Fabrication and efficient electromagnetic waves attenuation of three-dimensional porous reduced graphene oxide/boron nitride/silicon carbide hierarchical structures

doi:10.1016/j.jmst.2022.12.056

J. Mater. Sci. Technol. ›› 2023, Vol. 155: 192-201.DOI: 10.1016/j.jmst.2022.12.056

Fabrication and efficient electromagnetic waves attenuation of three-dimensional porous reduced graphene oxide/boron nitride/silicon carbide hierarchical structures

Qiuqi Zhang^a,b,c,1, Xiao You^b,c,1, Li Tian^b,c,d, Mengmeng Wang^b,c,d, Xiangyu Zhang^b,c, Ying Shi^a,*, Jinshan Yang^b,c,**, Shaoming Dong^b,c,e,**

^aSchool of Materials Science and Engineering, Shanghai University, Shanghai 200444, China;
^bState Key Laboratory of High Performance Ceramics & Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China;
^cStructural Ceramics and Composites Engineering Research Center, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China;
^dUniversity of Chinese Academy of Sciences, Beijing 100049, China;
^eCenter of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China

Received:2022-10-11 Revised:2022-11-27 Accepted:2022-12-25 Published:2023-08-20 Online:2023-03-04
Contact: **State Key Laboratory of High Performance Ceramics & Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sci-ences, Shanghai 200050, China. *E-mail addresses: yshi@shu.edu.cn (Y. Shi), jyang@mail.sic.ac.cn (J. Yang), smdong@mail.sic.ac.cn (S. Dong).
About author:¹These authors contributed equally to this work.

Abstract

Abstract: In this work, hierarchical hybrid composites consisting of porous three-dimensional reduced graphene oxide (3D-rGO) skeleton and lamellar boron nitride (BN)/silicon carbide (SiC) coatings are prepared by chemical vapor infiltration (CVI) process. The graphene framework prepared by 3D printing and frozen self-assembly exhibits a lightweight structure and a perforated conductive network, which extends the transmission path of incident microwaves. The introduced ceramic coatings can effectively tune the impedance matching degree and supply a lossy phase, and the hierarchical structure of the composites enhances the multiple scattering of the incident microwaves. As expected, the 3D-rGO/BN/SiC composites possess an excellent absorbing performance with a minimum reflection loss value of -37.8 dB, and the widest effective absorbing bandwidth (RL < -10 dB) of 5.90 GHz is obtained. The controllable fabrication of composites can provide a guideline for rational design and fabrication of high-performance electromagnetic waves absorbing materials in practical applications.

Key words: Porous network structure, Hierarchical structure, Electromagnetic wave absorbing, High attenuation ability, Effective absorbing bandwidth

Qiuqi Zhang, Xiao You, Li Tian, Mengmeng Wang, Xiangyu Zhang, Ying Shi, Jinshan Yang, Shaoming Dong. Fabrication and efficient electromagnetic waves attenuation of three-dimensional porous reduced graphene oxide/boron nitride/silicon carbide hierarchical structures[J]. J. Mater. Sci. Technol., 2023, 155: 192-201.

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Fabrication and efficient electromagnetic waves attenuation of three-dimensional porous reduced graphene oxide/boron nitride/silicon carbide hierarchical structures

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