J. Mater. Sci. Technol. ›› 2020, Vol. 45: 15-22.DOI: 10.1016/j.jmst.2019.09.040
• Research Article • Previous Articles Next Articles
Chao Wang*(), Qiang Li*(), Weiming Zhang, Huiqing Fan
Received:
2019-07-16
Revised:
2019-08-22
Accepted:
2019-09-12
Published:
2020-05-15
Online:
2020-05-27
Contact:
Chao Wang,Qiang Li
Chao Wang, Qiang Li, Weiming Zhang, Huiqing Fan. Large electric field-induced strain in the novel BNKTAN-BNBLTZ lead-free ceramics[J]. J. Mater. Sci. Technol., 2020, 45: 15-22.
Fig. 3. SEM images of BNKTAN-100xBNBLTZ ceramics: (a) x = 0; (b) x = 0.02; (c) x = 0.04; (d) x = 0.06. The insets show the corresponding average grain size distributions.
Fig. 5. Relative dielectric permittivity (εˊ) and loss tangent (tanδ) of BNKTAN-100xBNBLTZ ceramics at different frequencies (1 kHz, 10 kHz, and 100 kHz) and temperature (30-400 °C): (a) x = 0; (b) x = 0.02; (c) x = 0.04; (d) x = 0.06.
Compositions | Smax (%) | E (kV/cm) | d33* (pm/V) | Ref. |
---|---|---|---|---|
BNKTAN-0.04BNBLTZ | 0.505 | 65 | 777 | This work |
BNBT6.5-ES | 0.40 | 80 | 500 | [ |
92BNT-6BT-2KNN | 0.45 | 80 | 560 | [ |
BNT-BTN-2BSN | 0.40 | 60 | 669 | [ |
BNKTLa2-ST | 0.34 | 60 | 600 | [ |
BNBKL15 | 0.37 | 65 | 570 | [ |
BNKLTN-ST | 0.38 | 50 | 760 | [ |
BNKT-KNN | 0.46 | 80 | 575 | [ |
(BNT-BT-0.03ST)-LN | 0.44 | 55 | 800 | [ |
BNT-KT-22.5ST | 0.237 | 30 | 793 | [ |
Table 1 Contrast in strain performance of BNKTAN-0.04BNBLTZ ceramic with other BNT-based ceramics.
Compositions | Smax (%) | E (kV/cm) | d33* (pm/V) | Ref. |
---|---|---|---|---|
BNKTAN-0.04BNBLTZ | 0.505 | 65 | 777 | This work |
BNBT6.5-ES | 0.40 | 80 | 500 | [ |
92BNT-6BT-2KNN | 0.45 | 80 | 560 | [ |
BNT-BTN-2BSN | 0.40 | 60 | 669 | [ |
BNKTLa2-ST | 0.34 | 60 | 600 | [ |
BNBKL15 | 0.37 | 65 | 570 | [ |
BNKLTN-ST | 0.38 | 50 | 760 | [ |
BNKT-KNN | 0.46 | 80 | 575 | [ |
(BNT-BT-0.03ST)-LN | 0.44 | 55 | 800 | [ |
BNT-KT-22.5ST | 0.237 | 30 | 793 | [ |
Fig. 12. Fatigue properties of BNKTAN-4BNBLTZ ceramic sample: (a) unipolar strain at different cycles; (b) calculated maximum unipolar strain (S (%)) and d33* with the different switching cycles.
Fig. 13. (a) Complex AC impedance plots for BNKTAN-100xBNBLTZ ceramics (x = 0-0.06) tested at 993 K, (b) complex AC impedance plots of BNKTAN-4BNBLTZ at different temperatures, (c) Z″/Z″max and M″/M″max as a function of frequency for BNKTAN-4BNBLTZ ceramic measured at different temperature and (d) Arrhenius-type plots of bulk conductivity and activation energy for BNKTAN-100xBNBLTZ ceramics.
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