Enhanced capacitive energy storage and dielectric temperature stability of A-site disordered high-entropy perovskite oxides

doi:10.1016/j.jmst.2022.10.053

Abstract

Abstract: In this work, a novel high entropy perovskite oxide (1-x)(Na_0.2Bi_0.2Ba_0.2Sr_0.2Ca_0.2)TiO₃-xNaNbO₃ (abbreviated as (1-x)NBBSCT-xNN, x = 0, 0.05, 0.1, 0.15, and 0.2) was designed to improve temperature dielectric stability and energy storage performance by combining relaxor and antiferroelectric characteristics. The optimal composition of x = 0.2 exhibits a high energy storage density of 3.51 J/cm³, together with wide temperature stable stability ($\frac{C_T-C_{25^{\circ} \mathrm{C}}}{C_{25^{\circ} \mathrm{C}}}$< 15%, -70 to 110 °C), excellent frequency stability (W_rec and η vary by only ± 2.1% and ± 5.2% within the range of 1-600 Hz) and fast discharge rate (t_0.9 = 55.2 ns). This is mainly due to the enhancement of relaxation behavior and increase of E_b caused by the decrease of grain size. These results offer a new strategy for designing high entropy ceramic materials of high performance in the future.

Key words: Energy storage, High-entropy perovskite, Temperature stability, Relaxor ferroelectrics

Yating Ning, Yongping Pu, Chunhui Wu, Shiyu Zhou, Lei Zhang, Jinbo Zhang, Xian Zhang, Yangchao Shang. Enhanced capacitive energy storage and dielectric temperature stability of A-site disordered high-entropy perovskite oxides[J]. J. Mater. Sci. Technol., 2023, 145: 66-73.

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