J. Mater. Sci. Technol. ›› 2022, Vol. 104: 119-126.DOI: 10.1016/j.jmst.2021.06.048
• Research Article • Previous Articles Next Articles
Xudong Qia,b, Kai Lia, Enwei Suna,*(
), Bingqian Songc, Da Huoa, Jiaming Lic, Xianjie Wangc, Rui Zhanga,*(), Bin Yanga, Wenwu Caoa,d,*()
Received:2021-03-25
Revised:2021-06-21
Accepted:2021-06-27
Published:2022-03-30
Online:2021-09-08
Contact:
Enwei Sun,Rui Zhang,Wenwu Cao
About author:dzk@psu.edu (W. Cao).1 These authors contributed equally to this work.
Xudong Qi, Kai Li, Enwei Sun, Bingqian Song, Da Huo, Jiaming Li, Xianjie Wang, Rui Zhang, Bin Yang, Wenwu Cao. Large photovoltaic effect with ultrahigh open-circuit voltage in relaxor-based ferroelectric Pb(In1/2Nb1/2)O3-Pb(Mg1/3Nb2/3)O3-PbTiO3 ceramics[J]. J. Mater. Sci. Technol., 2022, 104: 119-126.
Fig. 1. (a) Phase diagram of ternary PIMN-PT system [36]. The selected composition is indicated by the green star. (b) XRD pattern of PIMN-34PT solid solutions. In the inset, the rhombohedral and tetragonal lattice structure schematic diagrams are shown. (c) SEM image of the PIMN-34PT sample. (d) The grain size distribution with Gaussian fitting of the selected samples.
Fig. 2. PFM images of the PIMN-34PT sample. (a) Surface topography image, (b) amplitude image, (c) phase image, (d) autocorrelation result and average autocorrelation function <C(r)> of the PIMN-34PT sample.
Fig. 3. (a) Temperature-dependent dielectric constant and dielectric loss of PIMN-34PT ceramics (0.5-50 kHz). (b) Hysteresis loops of PIMN-34PT ceramics under 5-40 kV/cm at room temperature. (c) UV-vis transmission spectrum of PIMN-34PT ceramics. Tauc plot ([F(R) hν]2 vs. hν) for bandgap calculations. The inset shows the transmission spectrum. (d) A summary of remnant polarization and bandgap of representative ferroelectric photovoltaic materials compared with those of PIMN-34PT ceramics. The data in Fig. 3(d) are extracted from Refs. [12,13,15].
Fig. 4. (a) Device with an architecture of ITO/PIMN-PT/Au under test. (b-d) Photocurrent responses for laser on/off cycles and polarization orientation of unpoling, positive poling, and negative poling states.
Fig. 5. (a) Current density-voltage (J-V) characteristics of PIMN-34PT ceramics. (b) Comparison bar diagram of Eoc of different ferroelectric crystals. sc = single crystal, bc = bulk ceramic. (c) J-V curves measured under different illumination intensities. (d) Schematic energy band graphs of ITO/PIMN-PT/Au devices under unpoling, positive poling, and negative poling states.
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