Controllable heterogeneous interfaces and dielectric regulation of hollow raspberry-shaped Fe3O4@rGO hybrids for high-performance electromagnetic wave absorption

doi:10.1016/j.jmst.2022.12.018

Abstract

Abstract: Heterogeneous interface engineering is closely related to the structural design of electromagnetic absorbers; thus, the interface control through structural design is a considerable approach to optimize the electromagnetic wave absorption (EWA) performance. Herein, the 3D hierarchical structure composites composed of two-dimensional reduced graphite oxide (rGO) and hollow raspberry Fe₃O₄ nanoparticles was successfully fabricated by a simple pyrolysis and self-assembly process. This specific structure enriches the characteristics of interface polarization and dipole polarization, which further induces significant EWA behavior. By adjusting the amount of graphite oxide (GO), the complex dielectric constant of the obtained hybrids can be controlled, and the heterointerface can be cleverly adjusted. The minimum reflection loss (RL_min) of the typical products can be up to -73.86 dB at the thickness is only 1.35 mm, and the maximum effective absorption bandwidth (EAB) can reach 5.1 GHz. This work demonstrates that the unique structure and tunable components can fully improve the potential of electromagnetic absorption performance, which provides basic guidance for the heterogeneous interface engineering of efficient electromagnetic functional materials.

Key words: Electromagnetic wave absorption, Dielectric regulation, Self-assemble, Hierarchical structure, Composites

Yuhan Wu, Shujuan Tan, Puyu Liu, Yan Zhang, Peng Li, Guangbin Ji. Controllable heterogeneous interfaces and dielectric regulation of hollow raspberry-shaped Fe₃O₄@rGO hybrids for high-performance electromagnetic wave absorption[J]. J. Mater. Sci. Technol., 2023, 151: 10-18.

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Controllable heterogeneous interfaces and dielectric regulation of hollow raspberry-shaped Fe₃O₄@rGO hybrids for high-performance electromagnetic wave absorption

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