J. Mater. Sci. Technol. ›› 2025, Vol. 222: 250-262.DOI: 10.1016/j.jmst.2024.04.088

• Research Article • Previous Articles     Next Articles

High-throughput production of low-cost hydrophobic and oleophilic mullite fiber sponges for high-temperature PM filtration

Yuwen Hua, Ruijian Zhub, Dazhi Zhenga, Shiou Lianga, Zengmei Wanga,*   

  1. aSchool of Materials Science and Engineering, Jiangsu Key lab. of Construction Materials, Southeast University, Nanjing 211189, China;
    bSchool of Materials Science and Engineering, Jiangsu Key Laboratory of Advanced Structural Materials and Application Technology, Nanjing Institute of Technology, Nanjing 211167, China
  • Received:2024-02-11 Revised:2024-04-23 Accepted:2024-04-24 Published:2025-07-01 Online:2024-10-16
  • Contact: * E-mail address: 101011338@seu.edu.cn (Z. Wang).

Abstract: Particulate matter (PM) from high-temperature emissions like chemical plants, coal stoves and vehicle exhausts poses a gravel challenge to human health. To address this issue, researchers have explored various fiber filters, yet the bulk struggle to withstand high temperatures. In this study, mullite fiber sponges were developed utilizing low-cost materials and Kármán vortex solution blow spinning, using surfactants to improve the spinnability of the sol. Optimized sponges demonstrate ultralight (19 mg cm-3), temperature-resistant reversible compressibility (50 % strain) and a water contact angle of 135°. These sponges exhibited exceptional thermal insulation (thermal conductivity: 0.0256 W m-1 K-1) and performed well in high-temperature air filtration. At 800 °C, the mullite sponge with a base weight of 35 mg cm-2, achieved an average filtration efficiency of 98.18 % and 99.57 % for PM2.5 and PM2.5-10, respectively, with a quality value of 0.98 Pa-1 at a wind speed of 4 cm s-1. This low-cost mullite fiber sponge offers a promising avenue for designing high-performance filtration materials.

Key words: Kármán vortex solution blow spinning, Mullite fiber, Thermal insulation, High-temperature PM filtration