J. Mater. Sci. Technol. ›› 2022, Vol. 123: 78-91.DOI: 10.1016/j.jmst.2021.12.076
• Research Article • Previous Articles Next Articles
Xiaoyun Qi, Shicheng Zhou, Hui Fang, Shuhan Yang, Chunjin Hang, Yanhong Tian, Chenxi Wang*()
Received:
2021-10-18
Revised:
2021-12-13
Accepted:
2021-12-21
Published:
2022-10-01
Online:
2022-09-30
Contact:
Chenxi Wang
About author:
*E-mail address: wangchenxi@hit.edu.cn (C.-X. Wang).Xiaoyun Qi, Shicheng Zhou, Hui Fang, Shuhan Yang, Chunjin Hang, Yanhong Tian, Chenxi Wang. One-step PDA coating strategy on pure Zn for blood-contacting engineering[J]. J. Mater. Sci. Technol., 2022, 123: 78-91.
Fig. 1. (a) Processing diagram of PDA coating on pure Zn surface process with solution stirred, (b) photographs of dopamine polymerization and solution absorbance at 420 nm in different pH dopamine-Tris solutions at various time.
Fig. 2. (a) Surface morphology SEM image of PDA coated Zn under pH=8.5 condition at various time, (b) cross-section SEM image and EDS mapping of PDA coated Zn under pH=8.5 condition, (c) surface morphology SEM image of PDA coated Zn under pH=10 condition at various time, (d) cross-section SEM image and EDS mapping of PDA coated Zn under pH=10.
Fig. 3. (a) Three-dimension surface topography image of pH 8.5 CG and pH 8.5 EG, (b) three-dimension surface topography image of pH 10 CG and pH 10 EG, (c) roughness comparison of different surface processing.
Fig. 4. C 1s, O 1s, N 1s and Zn 2p XPS spectra of (a) pure Zn surface, (b) pH=8.5 surface and (c) pH=10 surface; (d) FT-IR spectra and (e) Raman spectra of pH=8.5; (f) FT-IR spectra and (g) Raman spectra of pH=10.
Fig. 6. (a) Surface morphology and cross-section image of pure Zn, PDA-8.5, and PDA-10 during 28-day immersion degradation studies, (b) weight loss of different groups as a function of immersion time, (c) corrosion rate of different groups.
Fig. 7. (a) Potentiodynamic polarization curves of pure Zn, PDA-8.5 and PDA-10 in SBF solution, (b) Nyquist plots and fitting curves of different groups in SBF solution, (c) Bode plots of impedance vs. frenquency, (d) phase-frequency diagram, (e) equivalent circuits models of bare and coated samples.
Pure Zn | PDA-8.5 | PDA-10 | |
---|---|---|---|
Ecorr (V) | -1.17 | -1.15 | -1.14 |
icorr (μA cm-2) | 38.88 | 90.56 | 52.28 |
Table 1. Fitting results of the polarization curves
Pure Zn | PDA-8.5 | PDA-10 | |
---|---|---|---|
Ecorr (V) | -1.17 | -1.15 | -1.14 |
icorr (μA cm-2) | 38.88 | 90.56 | 52.28 |
Specimens | Pure Zn | PDA-8.5 | PDA-10 |
---|---|---|---|
Rs (Ω cm2) | 3.03 | 3.59 | 3.49 |
CPE1 (10-5 S cm-2 sn) | 3.85 | 2.78 | 1.24 |
n1 | 1.00 | 1.00 | 1.00 |
R1 (Ω cm2) | 31.44 | 107.34 | 92.70 |
CPE2 (10-5 S cm-2 sn) | 32.85 | 9.74 | 32.94 |
n2 | 0.76 | 0.70 | 0.47 |
R2 (Ω cm2) | 653.04 | 767.81 | 1569.55 |
W (10-3 S cm-2 s0.5) | 1.90 | - | - |
Table 2. Fitting results of EIS.
Specimens | Pure Zn | PDA-8.5 | PDA-10 |
---|---|---|---|
Rs (Ω cm2) | 3.03 | 3.59 | 3.49 |
CPE1 (10-5 S cm-2 sn) | 3.85 | 2.78 | 1.24 |
n1 | 1.00 | 1.00 | 1.00 |
R1 (Ω cm2) | 31.44 | 107.34 | 92.70 |
CPE2 (10-5 S cm-2 sn) | 32.85 | 9.74 | 32.94 |
n2 | 0.76 | 0.70 | 0.47 |
R2 (Ω cm2) | 653.04 | 767.81 | 1569.55 |
W (10-3 S cm-2 s0.5) | 1.90 | - | - |
Specimens | Rp (Ω) |
---|---|
Pure Zn | 686.38 |
PDA-8.5 | 875.15 |
PDA-10 | 1662.25 |
Table 3. Calculation of polarization resistance Rp.
Specimens | Rp (Ω) |
---|---|
Pure Zn | 686.38 |
PDA-8.5 | 875.15 |
PDA-10 | 1662.25 |
Fig. 8. (a) Hemolysis percentage, (b) APTT, PT, and TT, (c) FIB, (d) performance of adhered platelets, (e) platelets assembled number (per 2000× field) (n=3) of bare and coated samples. Statistically significant difference is indicated by *p < 0.05, **p < 0.005, using a one-way ANOVA.
Fig. 9. (a) SEM image and EDS mapping, (b) three-dimension morphology with roughness labelled, (c) PLGA coating thickness of pure Zn/PLGA, PDA-8.5/PLGA and PDA-10/PLGA composite coated structures.
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