Optimizing magnetic/dielectric matching in permalloy/carbonized cotton fiber composites by strain-tunable ferromagnetic resonance and defect-induced dielectric polarization

doi:10.1016/j.jmst.2022.01.027

Abstract

Abstract:

Electromagnetic losses in composites could be synergistically controlled by permeability and permittivity, associated with multiple ferromagnetic resonances and dielectric polarization. However, it is still challenging for simultaneous tunability for both the terms in a magnetic/dielectric composite system. Here, we demonstrate the tunable ferromagnetic resonances and the enhanced dielectric losses at gigahertz frequencies in permalloy/carbonized cotton fiber composites with different annealing temperatures. It is theoretically confirmed that the stress field acting on the magnetic permalloy layer increases with increasing temperature because of the shrinkage of the dielectric carbonized cotton fibers, resulting in multiple ferromagnetic resonances, in which there is a linear relationship (fr=1.52×σ+9.38) between the resonance frequency (f_r) and the stress (σ). The present work provides a fundamental insight into understanding the micromagnetic dynamics of the magnetic/dielectric composite system.

Key words: Ferromagnetic resonance, Stress tuning, Dielectric polarization

Xiaochen Shen, Chenglong Hu, Wenling Ren, Rongzhi Zhao, Lianze Ji, Xuefeng Zhang, Xinglong Dong. Optimizing magnetic/dielectric matching in permalloy/carbonized cotton fiber composites by strain-tunable ferromagnetic resonance and defect-induced dielectric polarization[J]. J. Mater. Sci. Technol., 2022, 124: 174-181.

Figures/Tables 8

Fig. 1. (a) Scheme of preparation of CC/Py and CCF/Pys. SEM images and elemental mapping of (b-f) CC/Py, (g-k) CCF/Py-200, (l-p) CCF/Py-300, and (q-u) CCF/Py-400.

Fig. 2. (a) Diameter statistics of the carbon fibers. (b) XRD spectra of the samples. (c) Lattice constant d and stress σ of CCF/Py-200, CCF/Py-300, and CCF/Py-400. (d) Schematic diagram of the stress on the magnetic permalloy layer.

Fig. 3. (a) Raman pattern of CC/Py, CCF/Py-200, CCF/Py-300, and CCF/Py-400; (b) corresponding defect concentration comparison.

Fig. 4. X-ray photoelectron spectroscopy analysis. High-resolution XPS survey of C element of (a) CC/Py, (b) CCF/Py-200, (c) CCF/Py-300 and (d) CCF/Py-400; (e) histogram of XPS survey of C element.

Fig. 5. Relative complex permeability at 8.2-12.4 GHz of (a) CC/Py, (b) CCF/Py-200, (c) CCF/Py-300, and (d) CCF/Py-400.

Fig. 6. (a) Real parts of relative complex permittivity and (b) imaginary parts of relative complex permittivity at 8.2-12.4 GHz of CC/Py, CCF/Py-200, CCF/Py-300, and CCF/Py-400.

Fig. 7. (a) Magnetic loss factor, (b) dielectric loss factor, (c) absorption coefficient A of CC/Py, CCF/Py-200, CCF/Py-300, CCF/Py-400.

Fig. 8. (a) Spatial magnetizations of the magnetic permalloy layer based on the strain-induced anisotropy constant (Keff). (b) Frequency dependence of the amplitude under different Keff. (c) Ferromagnetic resonance frequency fr varied with Keff.

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