J. Mater. Sci. Technol. ›› 2022, Vol. 118: 35-43.DOI: 10.1016/j.jmst.2021.11.059
• Research Article • Previous Articles Next Articles
Xi. Raoa,b,*(
), L. Dua,b, J.J. Zhaoa,b, X.D. Tana, Y.X. Fanga,b, L.Q. Xua,b, Y.P. Zhanga,*()
Received:2021-05-13
Revised:2021-10-20
Accepted:2021-11-09
Published:2022-08-10
Online:2022-02-22
Contact:
Xi. Rao,Y.P. Zhang
About author:zhangyyping@yahoo.com (Y.P. Zhang).Xi. Rao, L. Du, J.J. Zhao, X.D. Tan, Y.X. Fang, L.Q. Xu, Y.P. Zhang. Hybrid TiO2/AgNPs/g-C3N4 nanocomposite coatings on TC4 titanium alloy for enhanced synergistic antibacterial effect under full spectrum light[J]. J. Mater. Sci. Technol., 2022, 118: 35-43.
Fig. 1. SEM images of TC4 (a), HT-TC4 (b), 60Ag-TC4 (c), 0.5CN-TC4 (d), 0.5CN/60Ag-TC4 (e), and size distribution of AgNPs based on SEM images (f).
Fig. 2. SEM images and element mappings of 0.5CN/60Ag-TC4 (a), and line profile of Ti, Al, V, Ag, O, C, N (b).
Fig. 3. XRD patterns (a), Chemical composition of 0.5CN/60Ag-TC4 surface (b), and XPS spectra of C 1 s (c), N 1 s (d), Ti 2p (e), O 1 s (f), Ag 3d (g) for HT-TC4 and 0.5CN/60Ag-TC4.
Fig. 4. Biomedical properties of samples: hydrophilicity (a), cell proliferation (b) and cell viability (c).
Fig. 5. Antibacterial activity at dark and light irradiation against E. coli (a) and S. aureus (b).
Fig. 6. Long term antibacterial activity of 0.5CN/60Ag-TC4: SEM image of samples co-cultured with E. coli for different duration (a), and XPS survey scanning spectra (b), C 1 s spectra (c), Ti 2p spectra (d), Ag 3d spectra (e) of samples immersed in PBS for different duration.
Fig. 7. EPR spectra in the dark and under visible light irradiation, in methanol dispersion for DMAP-•O2- (a) and aqueous dispersion for DMAP-•OH, (b) for TiO2/AgNPs/g-C3N4 samples.
Fig. 8. Transient photocurrent responses (a), EIS spectra (b), UV-Vis absorbance spectra (c) and corresponding Kubelka-Munk transformed reflectance spectra (d).
Fig. 9. UPS spectra (a), Mott-Schottky curves (b), schematic illustration of band structure (c) of 0.5CN/60Ag-TC4, 0.5CN-TC4, and 60Ag-TC4, and photocatalytic antibacterial mechanism of TiO2/AgNPs/g-C3N4 heterojunction (d).
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