J. Mater. Sci. Technol. ›› 2022, Vol. 106: 139-146.DOI: 10.1016/j.jmst.2021.06.081
• Research Article • Previous Articles Next Articles
Yangfan Zhang, Yao Li, Han Yu*(), Kai Yu, Hongbing Yu
Received:
2021-02-26
Revised:
2021-06-28
Accepted:
2021-06-29
Published:
2022-04-20
Online:
2021-09-23
Contact:
Han Yu
About author:
*E-mail address: han.yu@tvrl.lth.se (H. Yu).Yangfan Zhang, Yao Li, Han Yu, Kai Yu, Hongbing Yu. Interfacial defective Ti3+ on Ti/TiO2 as visible-light responsive sites with promoted charge transfer and photocatalytic performance[J]. J. Mater. Sci. Technol., 2022, 106: 139-146.
Fig. 3. (a) HRTEM images of Ti/TiO2(1/10) with marked d-spacing and the corresponding fast Fourier transform (FFT) electron diffraction patterns (insets). The red square 1, 2 and 3 correspond to HRTEM of interface (b), HRTEM of Ti (c) and HRTEM of TiO2(d), respectively.
Fig. 4. (a) Ti 2p and (b) O 1s XPS spectra of the samples. (c) EPR spectra of the as-synthesized Ti/TiO2 samples. (d) The Raman spectra of TiO2 and Ti/TiO2(1/10).
Fig. 5. (a) The photodegradation activities and (b) the kinetic data curves of as-synthesized catalysts for photodegradation of RhB under visible light irradiation (λ > 420 nm). (c) The photocurrent of Ti/TiO2 samples under visible light irradiation (λ > 420 nm). (d) Recycling performance of Ti/TiO2(1/10) for RhB degradation under visible light.
Fig. 6. (a) PL spectra of Ti/TiO2 samples (excited at 250 nm). (b) TRPL spectra of the samples under an emission wavelength of 460 nm with an excitation wavelength of 250 nm.
Fig. 7. (a) XPS valence band spectra of TiO2 and Ti/TiO2(1/10). (b) The DOS plots of Ti, TiO2, and Ti/TiO2. (c) The 2D-ELF plots of TiO2, and Ti/TiO2 interface sliced along (101) plane of TiO2. (d) The proposed interfacial charge transfer mechanism on Ti/TiO2 photocatalysts.
[1] |
A. Fujishima, K. Honda, Bull. Chem. Soc. Jpn. 44 (1971) 1148-1150.
DOI URL |
[2] |
C.L. Wong, Y.N. Tan, A.R. Mohamed, J. Environ. Manage. 92 (2011) 1669-1680.
DOI URL |
[3] |
S.G. Kumar, L.G. Devi, J. Phys. Chem. A 115 (2011) 13211-13241.
DOI URL |
[4] |
V. Etacheri, C. Di Valentin, J. Schneider, D. Bahnemann, S.C. Pillai, J. Photochem. Photobiol. C-Photochem. Rev. 25 (2015) 1-29.
DOI URL |
[5] |
H. Tong, S. Ouyang, Y. Bi, N. Umezawa, M. Oshikiri, J. Ye, Adv. Mater. 24 (2012) 229-251.
DOI URL |
[6] |
J. Low, J. Yu, M. Jaroniec, S. Wageh, A. A. Al-Ghamdi, Adv. Mater. 29 (2017) 1601694.
DOI URL |
[7] |
A. Kumar, M. Khan, J. He, I.M.C. Lo, Water Res. 170 (2020) 115356.
DOI URL |
[8] |
A. Naldoni, M. Altomare, G. Zoppellaro, N. Liu, Š. Kment, R. Zbo ˇril, P. Schmuki, ACS Catal 9 (2019) 345-364.
DOI URL |
[9] |
S.G. Ullattil, S.B. Narendranath, S.C. Pillai, P. Periyat, Chem. Eng. J. 343 (2018) 708-736.
DOI URL |
[10] |
S. Chen, Y. Qi, C. Li, K. Domen, F. Zhang, Joule 2 (2018) 2260-2288.
DOI URL |
[11] |
J. Xiong, J. Di, J. Xia, W. Zhu, H. Li, Adv. Funct. Mater. 28 (2018) 1801983.
DOI URL |
[12] |
R. Shi, Y. Zhao, G.I.N. Waterhouse, S. Zhang, T. Zhang, ACS Catal 9 (2019) 9739-9750.
DOI URL |
[13] |
M. Xu, Y. Chen, J. Qin, Y. Feng, W. Li, W. Chen, J. Zhu, H. Li, Z. Bian, Environ. Sci. Technol. 52 (2018) 13879-13886.
DOI URL |
[14] |
Y. Chang, Y. Xuan, H. Quan, H. Zhang, S. Liu, Z. Li, K. Yu, J. Cao, Chem. Eng. J. 382 (2020) 122869.
DOI URL |
[15] |
J. Cai, M. Wu, Y. Wang, H. Zhang, M. Meng, Y. Tian, X. Li, J. Zhang, L. Zheng, J. Gong, Chem 2 (2017) 877-892.
DOI URL |
[16] |
W. Tu, Y. Zhou, Z. Zou, Adv. Mater. 26 (2014) 4607-4626.
DOI URL |
[17] |
G. Yin, X. Huang, T. Chen, W. Zhao, Q. Bi, J. Xu, Y. Han, F. Huang, ACS Catal 8 (2018) 1009-1017.
DOI URL |
[18] | Y.X. Zhao, Y.F. Zhao, R. Shi, B. Wang, G.I.N. Waterhouse, L.Z. Wu, C.H. Tung, T.R. Zhang, Adv. Mater. 31 (2019) 9. |
[19] |
F. Zuo, L. Wang, T. Wu, Z.Y. Zhang, D. Borchardt, P.Y. Feng, J. Am. Chem. Soc. 132 (2010) 11856-11857.
DOI URL |
[20] |
X. Chen, L. Liu, P.Y. Yu, S.S. Mao, Science 331 (2011) 746-750.
DOI URL |
[21] |
M.K. Nowotny, L.R. Sheppard, T. Bak, J. Nowotny, J. Phys. Chem. C 112 (2008) 5275-5300.
DOI URL |
[22] |
H.Q. Tan, Z. Zhao, M. Niu, C.Y. Mao, D.P. Cao, D.J. Cheng, P.Y. Feng, Z.C. Sun, Nanoscale 6 (2014) 10216-10223.
DOI URL |
[23] |
S. Liu, S. Yuan, Q. Zhang, B. Xu, C. Wang, M. Zhang, T. Ohno, J. Catal. 366 (2018) 282-288.
DOI URL |
[24] |
M. Kong, Y. Li, X. Chen, T. Tian, P. Fang, F. Zheng, X. Zhao, J. Am. Chem. Soc. 133 (2011) 16414-16417.
DOI URL |
[25] |
X. Yu, B. Kim, Y.K. Kim, ACS Catal 3 (2013) 2479-2486.
DOI URL |
[26] |
Y. Yan, M.Y. Han, A. Konkin, T. Koppe, D. Wang, T. Andreu, G. Chen, U. Vetter, J.R. Morante, P. Schaaf, J. Mater. Chem. A 2 (2014) 12708-12716.
DOI URL |
[27] |
H. Zhang, J. Cai, Y. Wang, M. Wu, M. Meng, Y. Tian, X. Li, J. Zhang, L. Zheng, Z. Jiang, J. Gong, Appl. Catal. B-Environ. 220 (2018) 126-136.
DOI URL |
[28] | X.Y. Xin, T. Xu, J. Yin, L. Wang, C.Y. Wang, Appl. Catal. B-Environ. 176 (2015) 354-362. |
[29] |
L.L. Hou, Z.J. Guan, T.F. Liu, C.Q. He, Q.Y. Li, J.J. Yang, Int. J. Hydrog. Energy 44 (2019) 8109-8120.
DOI URL |
[30] |
Q. Fu, W.-X. Li, Y. Yao, H. Liu, H.-Y. Su, D. Ma, X.-K. Gu, L. Chen, Z. Wang, H. Zhang, B. Wang, X. Bao, Science 328 (2010) 1141-1144.
DOI URL |
[31] |
K. Yu, L.-L. Lou, S. Liu, W. Zhou, Adv. Sci. 7 (2020) 1901970.
DOI URL |
[32] |
M.D. Segall, P.J.D. Lindan, M.J. Probert, C.J. Pickard, P.J. Hasnip, S.J. Clark, M.C. Payne, J. Phys.: Condens. Matter 14 (2002) 2717-2744.
DOI URL |
[33] |
G. Kresse, J. Furthmüller, Comput. Mater. Sci. 6 (1996) 15-50.
DOI URL |
[34] |
J.P. Perdew, K. Burke, M. Ernzerhof, Phys. Rev. Lett. 77 (1996) 3865-3868.
DOI PMID |
[35] |
P.E. Blöchl, Phys. Rev. B 50 (1994) 17953-17979.
DOI URL |
[36] |
G. Kresse, D. Joubert, Phys. Rev. B 59 (1999) 1758-1775.
DOI URL |
[37] |
H.J. Monkhorst, J.D. Pack, Phys. Rev. B 13 (1976) 5188-5192.
DOI URL |
[38] |
J.R. De Lile, S.G. Kang, Y.-A. Son, S.G. Lee, ACS Omega 4 (2019) 8056-8064.
DOI URL |
[39] |
Y. Zhou, C. Chen, N. Wang, Y. Li, H. Ding, J. Phys. Chem. C 120 (2016) 6116-6124.
DOI URL |
[40] |
H. Liu, D. Wang, L. Ji, J. Li, S. Liu, X. Liu, S. Jiang, J. Chromatogr. A 1217 (2010) 1898-1903.
DOI URL |
[41] | R.S. Guo, C.W. Wang, J.B. Chen, J. Wang, L.Q. Wang, W.M. Liu, Phys. B-Condens. Matter 405 (2010) 46 82-46 86. |
[42] |
S. Zhan, H. Zhang, Y. Zhang, Q. Shi, Y. Li, X. Li, Appl. Catal. B-Environ. 203 (2017) 199-209.
DOI URL |
[43] |
K. Yu, D. Lei, Y. Feng, H. Yu, Y. Chang, Y. Wang, Y. Liu, G.-C. Wang, L.-L. Lou, S. Liu, W. Zhou, J. Catal. 365 (2018) 292-302.
DOI URL |
[44] |
V.M. Khomenko, K. Langer, H. Rager, A. Fett, Phys. Chem. Miner. 25 (1998) 338-346.
DOI URL |
[45] |
S. Santangelo, G. Messina, G. Faggio, A. Donato, L. De Luca, N. Donato, A. Bonavita, G. Neri, J. Solid State Chem. 183 (2010) 2451-2455.
DOI URL |
[46] |
G. Zhu, J. Xu, W. Zhao, F. Huang, ACS Appl. Mater. Interfaces 8 (2016) 31716-31721.
DOI URL |
[47] |
A. Naldoni, M. Allieta, S. Santangelo, M. Marelli, F. Fabbri, S. Cappelli, C.L. Bianchi, R. Psaro, V. Dal Santo, J. Am. Chem. Soc. 134 (2012) 7600-7603.
DOI URL |
[48] |
G.S. Li, Z.C. Lian, X. Li, Y.Y. Xu, W.C. Wang, D.Q. Zhang, F.H. Tian, H.X. Li, J. Mater. Chem. A 3 (2015) 3748-3756.
DOI URL |
[49] |
C. Zhang, K. Yu, Y. Feng, Y. Chang, T. Yang, Y. Xuan, D. Lei, L.-L. Lou, S. Liu, Appl. Catal. B-Environ. 210 (2017) 77-87.
DOI URL |
[50] | M. Wen, J.H. Wang, R.F. Tong, D.N. Liu, H. Huang, Y. Yu, Z.K. Zhou, P.K. Chu, X.F. Yu, Adv. Sci. 6 (2019) 7. |
[51] | L.M. Liu, S.Q. Wang, H.Q. Ye, J. Mater. Sci. Technol. 19 (2003) 540-544. |
[1] | Zheng Zhang, Ying Huang, Xiang Li, Zhiming Zhou. Rational construction of hollow nanoboxes for long cycle life alkali metal ion batteries [J]. J. Mater. Sci. Technol., 2022, 102(0): 46-55. |
[2] | Bin Wang, Yuanfu Chen, Qi Wu, Yingjiong Lu, Xiaojuan Zhang, Xinqiang Wang, Bo Yu, DongXu Yang, Wanli Zhang. A co-coordination strategy to realize janus-type bimetallic phosphide as highly efficient and durable bifunctional catalyst for water splitting [J]. J. Mater. Sci. Technol., 2021, 74(0): 11-20. |
[3] | Zhengkun Xie, Xiaowei An, Zhijun Wu, Xiyan Yue, Jiajia Wang, Xiaogang Hao, Abuliti Abudula, Guoqing Guan. Fluoropyridine family: Bifunction as electrolyte solvent and additive to achieve dendrites-free lithium metal batteries [J]. J. Mater. Sci. Technol., 2021, 74(0): 119-127. |
[4] | Sheng Guo, Zhixiong Yang, Huali Zhang, Wei Yang, Jun Li, Kun Zhou. Enhanced photocatalytic degradation of organic contaminants over CaFe2O4 under visible LED light irradiation mediated by peroxymonosulfate [J]. J. Mater. Sci. Technol., 2021, 62(0): 34-43. |
Viewed | ||||||
Full text |
|
|||||
Abstract |
|
|||||