2D Ti3C2Tx modifie d with nano-AgPNPs antioxidant constructed hierarchical interface for high-throughput oily wastewater separation

doi:10.1016/j.jmst.2023.10.039

Abstract

Abstract: Over-exploitation of fossil energy has led to the formation of enormous amounts of oily wastewater, which is increasingly polluting the environment of water bodies. The Ti₃C₂T_x-modified separation material is limited by surface roughness and surface chemical composition, and the permeation flux decreases significantly during continuous testing. In this study, silver-loaded polydopamine nanospheres (nano-AgPNPs) as antioxidants were prepared by in-situ reduction from Ag⁺ ions and polydopamine nanospheres, and then they self-assembled with Ti₃C₂T_x nanosheets to obtain hierarchical micro-nano structural nano-AgPNPs modified Ti₃C₂T_x [(AgPNPs)_xT (x = 0.25, 0.5, 0.75, and 1)]. Because of their strong reduction properties, nano-AgPNPs antioxidants can effectively protect the active edges of Ti₃C₂T_x from dissolved oxygen, and greatly improve the oxidation resistance of Ti₃C₂T_x nanosheets, with no significant changes in morphology and physical phase after long-term placement. (AgPNPs)_xT formed underwater oleophobic interfaces with the hierarchical structure on polyurethane (PU) sponge to prepare (AgPNPs)_xT@PU separation sponges. Among them, (AgPNPs)_0.5T@PU sponge showed the highest comprehensive performance with separation efficiency higher than 99.6% for various oil-water mixtures, especially high-throughput and permeation flux up to 247,787 L m^-2 h^-1 for cyclohexane-water mixtures. In addition, nano-AgPNPs greatly broadened the layer spacing of Ti₃C₂T_x and can form a functionalized interface of modified Ti₃C₂T_x on polyamide (PA) membrane and provide additional permeation channels, which enabled the (AgPNPs)_0.5T@PA membrane to have excellent toluene-water emulsion separation efficiency up to 99.6%.

Key words: Ti₃C₂T_x, Nano-AgPNPs, High-throughput, Oily wastewater separation, Oxidation resistance

Qing-Ming Wang, Xu-Han Chen, Qiu-Feng Lü, Qilang Lin. 2D Ti₃C₂T_x modifie d with nano-AgPNPs antioxidant constructed hierarchical interface for high-throughput oily wastewater separation[J]. J. Mater. Sci. Technol., 2024, 185: 133-146.

References

[1] G. Shi, M. Wu, Q. Zhong, P. Mu, J. Li, Langmuir 37 (2021) 7843-7850.
[2] H. Li, Q. Zhong, Q. Sun, B. Xiang, J. Li, Langmuir 38 (2022) 3493-3500.
[3] S. Gan, H. Li, X. Zhu, X. Liu, K. Wei, L. Zhu, B. Wei, X. Luo, J. Zhang, Q. Xue, Adv. Funct. Mater. 33 (2023) 2305975.
[4] H. Li, Y. Yin, L. Zhu, Y. Xiong, X. Li, T. Guo, W. Xing, Q. Xue, J. Hazard. Mater. 373 (2019) 725-732.
[5] H. Li, J. Zhang, S. Gan, X. Liu, L. Zhu, F. Xia, X. Luo, Q. Xue, Adv. Funct. Mater. 33 (2023) 2212582.
[6] X. Zhu, Z. Gao, F. Li, G. Miao, T. Xu, X. Miao, Y. Song, X. Li, G. Ren, Carbon 190 (2022) 329-336.
[7] Y. Cheng, Y. Cai, Z. Wang, X. Lu, H. Xia, Chem. Eng. J. 430 (2022) 132894.
[8] A. Chen, H. Guo, J. Zhou, Y. Li, X. He, L. Chen, Y. Zhang, A.C.S.Appl, Nano Mater. 5 (2022) 3925-3936.
[9] X. Jia, M. Peydayesh, Q. Huang, R. Mezzenga, Small 18 (2022) 2105502.
[10] A.S. Levitt, M. Alhabeb, C.B. Hatter, A. Sarycheva, G. Dion, Y. Gogotsi, J. Mater. Chem. A 7 (2019) 269-277.
[11] X.-D. Zhu, Y. Xie, Y.-T. Liu, J. Mater. Chem. A 6 (2018) 21255-21260.
[12] K. Li, G. Zou, T. Jiao, R. Xing, L. Zhang, J. Zhou, Q. Zhang, Q. Peng, Colloids Surf. A-Physicochem. Eng.Asp. 553 (2018) 105-113.
[13] J. Yin, L. Zhang, T. Jiao, G. Zou, Z. Bai, Y. Chen, Q. Zhang, M. Xia, Q. Peng, Nanomaterials 9 (2019) 1009.
[14] S. Wang, S. Wei, S. Wang, X. Zhu, C. Lei, Y. Huang, Z. Nie, S. Yao, Anal. Chem. 91 (2019) 1651-1658.
[15] S. He, Y. Zhan, J. Hu, G. Zhang, S. Zhao, Q. Feng, W. Yang, Compos. B-Eng. 197 (2020) 108188.
[16] S. Zhou, L. Xie, M. Yan, H. Zeng, X. Zhang, J. Zeng, Q. Liang, T. Liu, P. Chen, L. Jiang, B. Kong, Analyst 147 (2022) 652-660.
[17] Q.-M. Wang, Z.-H. Liu, Q.-F. Lü, Colloids Surf. A-Physicochem. Eng. Asp. 656 (2023) 130371.
[18] Z.-H. Liu, Q.-M. Wang, Q.-F. Lü, J. Wu, Colloids Surf. A-Physicochem. Eng. Asp. 640 (2022) 128396.
[19] S. Gu, Y. Ma, T. Zhang, Y. Yang, Y. Xu, J. Li, ACS EST Water 3 (2023) 1756-1766.
[20] H.A. Lee, Y. Ma, F. Zhou, S. Hong, H. Lee, Acc. Chem. Res. 52 (2019) 704-713.
[21] K. Ai, Y. Liu, C. Ruan, L. Lu, G. (Max) Lu, Adv.Mater. 25 (2013) 998-1003.
[22] X. Yu, H. Fan, L. Wang, Z. Jin, Angew. Chem. Int. Ed. 53 (2014) 12600-12604.
[23] J. Lu, J. Fang, J. Li, C. Wang, Z. He, L. Zhu, Z. Xu, H. Zeng, A.C.S.Appl, Nano Mater. 3 (2020) 156-164.
[24] C. Wu, G. Zhang, T. Xia, Z. Li, K. Zhao, Z. Deng, D. Guo, B. Peng, Mater. Sci. Eng. C 55 (2015) 155-165.
[25] N. Mehranbod, M. Khorram, S. Azizi, N. Khakinezhad, J. Environ. Chem.Eng. 9 (2021) 106245.
[26] J. Dai, L. Wang, Y. Wang, S. Tian, X. Tian, A. Xie, R. Zhang, Y. Yan, J. Pan, ACS Appl. Mater. Interfaces 12 (2020) 4 482-4 493.
[27] V. Natu, M. Clites, E. Pomerantseva, M.W. Barsoum, Mater. Res. Lett. 6 (2018) 230-235.
[28] Mu. Naushad, T. Ahamad, B.M. Al-Maswari, A.Abdullah Alqadami, S.M. Alshehri, Chem. Eng. J. 330 (2017) 1351-1360.
[29] Q. Xu, B. Zong, Q. Li, X. Fang, S. Mao, K. (Ken) Ostrikov, J.Hazard. Mater. 424 (2022) 127492.
[30] H. Riazi, M. Anayee, K. Hantanasirisakul, A.A. Shamsabadi, B. Anasori, Y. Gogotsi, M. Soroush, Adv. Mater. Interfaces 7 (2020) 1902008.
[31] Z. Ghelichkhah, S. Sharifi-Asl, K. Farhadi, S. Banisaied, S. Ahmadi, D.D. Macdonald, Corros. Sci. 91 (2015) 129-139.
[32] S. Sun, X. Sha, J. Liang, G. Yang, X. Hu, Y. Wen, M. Liu, N. Zhou, X. Zhang, Y. Wei, J. Colloid Interface Sci. 601 (2021) 294-304.
[33] Q.-M. Wang, J.-C. Lin, Z.-H. Liu, Q.-F. Lü, Ceram. Int. 49 (2023) 17437.
[34] R. Jin, X. Jiang, Y. Zhou, J. Zhao, Chin. J. Catal. 37 (2016) 760-768.
[35] Y. Zhou, M. Liu, Y. Wang, J. Yuan, X. Men, Tribol. Int. 165 (2022) 107328.
[36] W. Luo, Z. Niu, P. Mu, J. Li, Macromolecules 55 (2022) 9851-9859.
[37] C.J. Zhang, S. Pinilla, N. McEvoy, C.P. Cullen, B. Anasori, E. Long, S.-H. Park, A. Seral-Ascaso, A. Shmeliov, D. Krishnan, C. Morant, X. Liu, G.S. Duesberg, Y. Gogotsi, V. Nicolosi, Chem. Mater. 29 (2017) 4 84 8-4 856.
[38] R. Gulfam, P. Zhang, Colloids Surf. A Physicochem.Eng. Asp. 625 (2021) 126883.
[39] O. Mashtalir, K.M. Cook, V.N. Mochalin, M. Crowe, M.W. Barsoum, Y. Gogotsi, J. Mater. Chem. A 2 (2014) 14334-14338.
[40] Z. Wang, J. Guo, J. Ma, L. Shao, J. Mater. Chem. A 3 (2015) 19960-19968.
[41] Y.-F. Deng, D.Zhang, N. Zhang, T. Huang, Y.-Z. Lei, Y. Wang, J. Hazard. Mater. 407 (2021) 124787.
[42] C. Chen, D. Weng, A. Mahmood, S. Chen, J. Wang, ACS Appl. Mater. Interfaces 11 (2019) 11006-11027.
[43] H. Cao, Y. Liu, J. Colloid Interface Sci. 598 (2021) 4 83-4 91.
[44] C. Ma, L. Zhu, X. Qiao, H. Li, X. Zhu, J. Xue, Q. Xue, Surf. Coat. Technol. 406 (2021) 126642.
[45] D.-L. Zhou, D.Yang, D. Han, Q. Zhang, F. Chen, Q. Fu, J. Membr. Sci. 620 (2021) 118898.
[46] X. Yin, Y. He, T. He, H. Li, J. Wu, L. Zhou, S. Li, C. Li, Colloids Surf. A-Physicochem. Eng.Asp. 657 (2023) 130515.
[47] W. Wang, S. Jiao, B. Wang, Y. Tan, Y. Zhao, Q. Zhang, Y. Kang, X. Lv, C. Cui, G. Pang, Appl. Surf. Sci. 570 (2021) 151128.
[48] P. Song, Q. Lu, Sep. Purif. Technol. 238 (2020) 116454.
[49] M. Faraji, S.R. Nabavi, H. Salimi-Kenari, New J. Chem. 44 (2020) 13488-13500.
[50] C. Du, G. Liu, Z. Qu, W. Wang, D. Yu, J. Mater. Sci. 57 (2022) 3452-3467.
[51] J. Ge, Q. Jin, D. Zong, J. Yu, B. Ding, ACS Appl. Mater. Interfaces 10 (2018) 16183-16192.
[52] Y. Li, Y. He, J. Zhuang, H. Shi, Colloids Surf. A-Physicochem. Eng.Asp. 634 (2022) 128041.
[53] J. Wu, Z. Hou, Z. Yu, J. Lang, J. Cui, J. Yang, J. Dai, C. Li, Y. Yan, A. Xie, Sep. Purif. Technol. 258 (2021) 118022.
[54] Y. Gu, B. Zhang, Z. Fu, J. Li, M. Yu, L. Li, J. Li, J. Membr. Sci. 619 (2021) 118792.
[55] M. Tian, Y. Liao, R. Wang, J. Membr. Sci. 596 (2020) 117721.
[56] H. Zhan, T. Zuo, R. Tao, C. Chang, A.C.S.Sustain, Chem. Eng. 6 (2018) 10833-10840.

2D Ti₃C₂T_x modifie d with nano-AgPNPs antioxidant constructed hierarchical interface for high-throughput oily wastewater separation

PDF (PC)

Knowledge

Abstract

Cite this article

share this article

References

Related Articles 15

Recommended Articles

Metrics

Comments

[1]	Haoran Sun, Zhigang Ding, Hao Sun, Junjun Zhou, Ji-Chang Ren, Qingmiao Hu, Wei Liu. An efficient scheme for accelerating the calculation of stacking fault energy in multi-principal element alloys [J]. J. Mater. Sci. Technol., 2024, 175(0): 204-211.
[2]	T.S. Liang, Y.F. Jiang, H.Y. Li, W. Wang, Q. Zhang, B. Zhang. Enhanced oxidation resistance of Ce by addition of Ga and nanocrystallization [J]. J. Mater. Sci. Technol., 2023, 147(0): 26-36.
[3]	Rui Ma, Xiping Guo. Cooperative effects of Mo, V and Zr additions on the microstructure and properties of multi-elemental Nb-Si based alloys [J]. J. Mater. Sci. Technol., 2023, 132(0): 27-41.
[4]	Zhichao Lu, Yibo Zhang, Wenyue Li, Jinyue Wang, Xiongjun Liu, Yuan Wu, Hui Wang, Dong Ma, Zhaoping Lu. Materials genome strategy for metallic glasses [J]. J. Mater. Sci. Technol., 2023, 166(0): 173-199.
[5]	Guangyu Han, Wei Zhu, Siming Guo, Jie Zhou, Yutong Liu, Yuan Deng. Combinatorial screening via high-throughput preparation: Thermoelectric performance optimization for n-type Bi-Te-Se film with high average zT > 1 [J]. J. Mater. Sci. Technol., 2023, 160(0): 18-27.
[6]	L. Zhao, L. Jiang, L.X. Yang, H. Wang, W.Y. Zhang, G.Y. Ji, X. Zhou, W.A. Curtin, X.B. Chen, P.K. Liaw, S.Y. Chen, H.Z. Wang. High throughput synthesis enabled exploration of CoCrFeNi-based high entropy alloys [J]. J. Mater. Sci. Technol., 2022, 110(0): 269-282.
[7]	Lei Zhou, Jiaping Zhang, Dou Hu, Qiangang Fu, Wuqing Ding, Jiaqi Hou, Bing Liu, Mingde Tong. High temperature oxidation and ablation behaviors of HfB₂-SiC/SiC coatings for carbon/carbon composites fabricated by dipping-carbonization assisted pack cementation [J]. J. Mater. Sci. Technol., 2022, 111(0): 88-98.
[8]	Heguang Liu, Zhe Wang, Yujia Yang, Shaoqing Wu, Chukai Wang, Caiyin You, Na Tian. Thermally conductive MWCNTs/Fe₃O₄/Ti₃C₂T_x MXene multi-layer films for broadband electromagnetic interference shielding [J]. J. Mater. Sci. Technol., 2022, 130(0): 75-85.
[9]	Kunpeng Qian, Shuang Li, Jianhui Fang, Yuhuan Yang, Shaomei Cao, Miao Miao, Xin Feng. C₆₀ intercalating Ti₃C₂T_x MXenes assisted by γ-cyclodextrin for electromagnetic interference shielding films with high stability [J]. J. Mater. Sci. Technol., 2022, 127(0): 71-77.
[10]	Zhuojie Shao, Zhen Wu, Luchao Sun, Xianpeng Liang, Zhaoping Luo, Haikun Chen, Junning Li, Jingyang Wang. High entropy ultra-high temperature ceramic thermal insulator (Zr_1/5Hf_1/5Nb_1/5Ta_1/5Ti_1/5)C with controlled microstructure and outstanding properties [J]. J. Mater. Sci. Technol., 2022, 119(0): 190-199.
[11]	Yunli Lu, Fenghui Duan, Jie Pan, Yi Li. High-throughput screening of critical size of grain growth in gradient structured nickel [J]. J. Mater. Sci. Technol., 2021, 82(0): 33-39.
[12]	Jia Li, Baobin Xie, Qihong Fang, Bin Liu, Yong Liu, Peter K. Liaw. High-throughput simulation combined machine learning search for optimum elemental composition in medium entropy alloy [J]. J. Mater. Sci. Technol., 2021, 68(0): 70-75.
[13]	Jianping Lai, Wen Hu, Amit Datye, Jingbei Liu, Jan Schroers, Udo D. Schwarz, Jiaxin Yu. Revealing the relationships between alloy structure, composition and plastic deformation in a ternary alloy system by a combinatorial approach [J]. J. Mater. Sci. Technol., 2021, 84(0): 97-104.
[14]	Zejiang Yu, Wei Zheng, Zhiqiang Li, Yunzhuo Lu, Xinbing Yun, Zuoxiang Qin, Xing Lu. Accelerated exploration of TRIP metallic glass composite by laser additive manufacturing [J]. J. Mater. Sci. Technol., 2021, 78(0): 68-73.
[15]	Kunming Pan, Yanping Yang, Shizhong Wei, Honghui Wu, Zhili Dong, Yuan Wu, Shuize Wang, Laiqi Zhang, Junping Lin, Xinping Mao. Oxidation behavior of Mo-Si-B alloys at medium-to-high temperatures [J]. J. Mater. Sci. Technol., 2021, 60(0): 113-127.