lerating the design of multicomponent rare earth silicates for SiCf/SiC CMC by combinatorial material chip design and high throughput screening

doi:10.1016/j.jmst.2022.11.043

Abstract

Abstract: High throughput experimentation is employed to establish a ternary system with the compositional range of 30.8 mol.%-75.7 mol.% SiO₂, 16.6 mol.%-61.7 mol.% Yb₂O₃, and 6.3 mol.%-14.1 mol.% Ho₂O₃ through co-sputtering deposition on one combinatorial material chip. Considering their application in advanced SiC_f/SiC CMC, the phase composition and mechanical properties of samples with various RE/Si ratios and Yb/Ho ratios are comprehensively investigated. Chemical stability and thermal expansion compatibility between SiC and RE silicates with different compositions are also validated. Optimized materials for the application of environmental barrier coating and interphase for SiC_f/SiC CMC are screened respectively according to the above trends and data. This work is a case study to establish a composition-property library for RE₂O₃-SiO₂ compounds. It is inspired more complicated multicomponent RE silicates could be prepared and characterized by high throughput experimentation, accelerating the design and screening of promising optimal candidates.

Key words: High throughput experimentation, RE silicates, Phase stability, Mechanical properties

Xirui Lv, Yiming Lei, Zhao Zhang, Jie Zhang, Jingyang Wang. lerating the design of multicomponent rare earth silicates for SiC_f/SiC CMC by combinatorial material chip design and high throughput screening[J]. J. Mater. Sci. Technol., 2023, 150: 96-103.

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lerating the design of multicomponent rare earth silicates for SiC_f/SiC CMC by combinatorial material chip design and high throughput screening

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