Magnetic resonance behavior modulation of Ba3Co1.6-xZnxCu0.4Fe24O41 hexaferrites for microwave absorption and surface wave suppression

doi:10.1016/j.jmst.2024.06.048

Abstract

Abstract: The intrinsic high magnetocrystalline anisotropy equivalent field can help the hexaferrites break through Snoek's limit and increase the resonance frequency. This is advantageous for microwave absorption applications in the mid to low-frequency range of gigahertz. In this study, we prepared Z-type Ba₃Co_1.6-_xZn_xCu_0.4Fe₂₄O₄₁ hexaferrites using the sol-gel auto-combustion method. By changing the ratio of Co and Zn ions, the magnetocrystalline anisotropy of ferrite is further manipulated, resulting in significant changes in their magnetic resonance frequency and intensity. Ba₃Zn_1.6Cu_0.4Fe₂₄O₄₁ with high-frequency resonance achieved the lowest reflectivity of -72.18 dB at 15.56 GHz, while Ba₃Co_1.5Zn_0.1Cu_0.4Fe₂₄O₄₁ with stronger loss obtained the widest bandwidth of 4.93 GHz (6.14-11.07). Additionally, we investigated surface wave suppression properties previously overlooked. Ba₃Co_1.5Zn_0.1Cu_0.4Fe₂₄O₄₁ can achieve a larger attenuation at low frequency under low thickness, which has an excellent effect on reducing backscattering. This work provides a useful reference for the preparation and application of high-performance magnetic-loss materials.

Key words: Ferrite, Permeability, Microwave absorption, Surface wave

Ruiyang Tan, Liqiang Jin, Xuyao Wei, Bo Wei, Jintang Zhou, Ping Chen. Magnetic resonance behavior modulation of Ba₃Co_1.6-_xZn_xCu_0.4Fe₂₄O₄₁ hexaferrites for microwave absorption and surface wave suppression[J]. J. Mater. Sci. Technol., 2025, 214: 292-301.

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Magnetic resonance behavior modulation of Ba₃Co_1.6-_xZn_xCu_0.4Fe₂₄O₄₁ hexaferrites for microwave absorption and surface wave suppression

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