Effective CO2 activation of enriched oxygen vacancies for photothermal CO2 methanation

doi:10.1016/j.jmst.2023.11.068

Abstract

Abstract: Oxygen vacancies have been widely concerned with the facilitation effects of CO₂ activation for CO₂ methanation. However, little attention has been paid to the generation of active intermediate species induced by enriched oxygen vacancies. Herein, we discovered that CeNiO_3-_δ catalyst enriched oxygen vacancies can efficiently activate CO₂ and realize high activity for photothermal CO₂ methanation. In situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) proved that oxygen vacancies are beneficial to the formation of reactive intermediate species of polydentate carbonate over CeNiO_3-_δ, which is crucial for efficient CO₂ methanation. These results revealed mechanistic insights into how effective CO₂ activation induced by oxygen vacancies can be manipulated by adjusting the adsorption intermediate species.

Key words: Oxygen vacancies, CO₂ activation, Active intermediate species, Photo-thermal CO₂ methanation, CeNiO₃

Peipei Du, Guoqiang Deng, Zhonghua Li, Junchuan Sun, Lu Wang, Yongqiang Yang, Jun Wang, Yaguang Li, Xiaoming Xu, Yuanming Zhang, Wangxi Liu, Gang Liu, Zhigang Zou, Zhaosheng Li. Effective CO₂ activation of enriched oxygen vacancies for photothermal CO₂ methanation[J]. J. Mater. Sci. Technol., 2024, 189: 203-210.

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Effective CO₂ activation of enriched oxygen vacancies for photothermal CO₂ methanation

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