Construction of one-dimensional hierarchical MoS2/Ni3S2 composites with enhanced interfacial polarization and improved wideband microwave absorption

doi:10.1016/j.jmst.2023.08.044

Abstract

Abstract: The construction of one-dimensional (1D) sulfides has attracted extensive attention for improving microwave absorption (MA) performance owing to the anisotropic conductive networks. However, the synthesis of conductive 1D hierarchical materials with unique interfacial polarization and excellent MA properties remains challenging. In this study, cable-like MoS₂/Ni₃S₂ was synthesized by a one-step hydrothermal strategy. The complex permittivity of the binary composites could be improved by tuning the thickness of the MoS₂ coating. Importantly, the construction of heterogeneous contacts by MoS₂ and Ni₃S₂ contributed to enhanced polarization loss, and the charge distribution was validated by electron holography. The wide efficient absorption bandwidth can reach above 4.8 GHz at a thin thickness. These new discoveries shed light on novel structures for 1D sulfide materials and the design of functional core-shell composites for microwave absorption.

Key words: 1D sulfide materials, Microwave absorption, MoS₂/Ni₃S₂, Interfacial polarization, Core-shell composites

Kaicheng Luo, Biao Zhao, Chunyang Xu, Chongyun Liang, Chang Zhang, Yiqian Du, Xiaowei Lv, Jincang Zhang, Limin Wu, Renchao Che. Construction of one-dimensional hierarchical MoS₂/Ni₃S₂ composites with enhanced interfacial polarization and improved wideband microwave absorption[J]. J. Mater. Sci. Technol., 2024, 178: 22-28.

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Construction of one-dimensional hierarchical MoS₂/Ni₃S₂ composites with enhanced interfacial polarization and improved wideband microwave absorption

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