Hollow engineering of sandwich NC@Co/NC@MnO2 composites toward strong wideband electromagnetic wave attenuation

doi:10.1016/j.jmst.2023.08.020

Abstract

Abstract: Multiple hetero-interfaces would strengthen interfacial polarization and boost electromagnetic wave absorption, but still remain the formidable challenges in decreasing filler loadings. Herein, sandwich NC@Co/NC@MnO₂ composites with hollow cavity, multiple hetero-interfaces, and hierarchical structures have been fabricated via the cooperative processes of self-sacrifice strategy and sequential hydrothermal reaction. In the sandwich composites, middle magnetic components (Co/NC) are wrapped by inner N-doped carbon (NC) matrix and outer hierarchical MnO₂ nanosheets. Importantly, hollow engineering of sandwich composites with multiple hetero-interfaces greatly facilitates the enhancement of absorption bandwidth without sacrificing the absorption intensity. The maximum reflection loss of sandwich NC@Co/NC@MnO₂ composites reaches -44.8 dB at 2.5 mm and the effective bandwidths is achieved as wide as 9.6 GHz at 2.3 mm. These results provide us a new insight into preparing efficient electromagnetic wave absorbers by interface engineering and hollow construction.

Key words: Interface engineering, Sandwich structure, Hetero-interfaces, Interfacial polarization, Electromagnetic wave absorption

Chenhao Wei, Lingzi Shi, Maoqing Li, Mukun He, Mengjie Li, Xinrui Jing, Panbo Liu, Junwei Gu. Hollow engineering of sandwich NC@Co/NC@MnO₂ composites toward strong wideband electromagnetic wave attenuation[J]. J. Mater. Sci. Technol., 2024, 175: 194-203.

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Hollow engineering of sandwich NC@Co/NC@MnO₂ composites toward strong wideband electromagnetic wave attenuation

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