Organic interlayer engineering of TiS2 for enhanced aqueous Zn ions storage

doi:10.1016/j.jmst.2022.09.012

Abstract

Abstract: Aqueous rechargeable zinc-ion batteries (ARZIBs) have a bright future for energy storage due to their high energy density and safety. However, for traditional ARZIBs, cathode materials always suffer from the limited space for large-sized zinc ions storage and transport, leading to low Coulombic efficiency and inferior cycling performance. To build a reliable host with large tunnel, 1-butyl-1-methylpyrrolidinium ion (PY14⁺) pre-intercalated TiS₂ (PY14⁺-TiS₂) is designed as an alternative intercalation-type electrode. As the insertion organic guest widens the interlayer space of TiS₂ and buffers the lattice stress generated during the electrochemical cycles, the structural reversibility, cycling stability and kinetics properties of PY14⁺-TiS₂ are enhanced greatly. A specific capacity of 130.9 mAh g^-1 with 84.3% capacity retention over 500 cycles can be achieved at 0.1 A g^-1. Therefore, this study paves the way for enhancing the aqueous Zn ions storage capability by organic interlayer engineering.

Key words: Pre-intercalation, Organic interlayer engineering, TiS₂, Intercalation-type electrode, Aqueous zinc-ion batteries

Chengcheng Huang, Yiwen Liu, Jing Li, Zhonghao Miao, Xinhao Cai, Zhouxiang Wu, Haoxiang Yu, Lei Yan, Liyuan Zhang, Jie Shu. Organic interlayer engineering of TiS₂ for enhanced aqueous Zn ions storage[J]. J. Mater. Sci. Technol., 2023, 140: 135-141.

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Organic interlayer engineering of TiS₂ for enhanced aqueous Zn ions storage

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