An embedded ReS2@MAPbBr3 heterostructure with downhill interfacial charge transfer for photocatalytic upgrading of biomass-derived alcohols to aldehydes and H2

doi:10.1016/j.jmst.2023.08.009

Abstract

Abstract: Solar-driven selective upgrading of lignocellulosic biomass-derived alcohols to value-added chemicals and clean fuel hydrogen (H₂) shows great potential for tackling the energy crisis and environmental pollution issues. Here, we construct a MAPbBr₃/ReS₂ heterostructure by embedding distorted tetragonal (1T) phase ReS₂ nanoflowers into large-sized MAPbBr₃ for green value-added utilization of biomass-derived alcohols. The embedded structure effectively enlarges the contact interface between the ReS₂ and the MAPbBr₃, and importantly, induces a strong built-in electric field aligned between the spatially well-defined MAPbBr₃ and ReS₂ nanoflowers. Moreover, the distorted 1T phase ReS₂ with low work function well matches the energy band of MAPbBr₃, forming a heterostructure with a downward band bending at the interface. These features empower the MAPbBr₃/ReS₂ photocatalyst with high capability to promote charge separation and expedite the surface redox reaction. Consequently, optimal BAD and H₂ production rates of about 1220 μmol h^-1 g^-1 are realized over a MAPbBr₃/ReS₂ 2% sample, which are approximately 9 times greater than those of blank MAPbBr₃. This work demonstrates the great potential of constructing an embedded transition metal dichalcogenide@metal halide perovskites heterostructure with downhill interfacial charge transfer for photocatalytic upgrading of biomass-derived alcohols.

Key words: Heterostructure, Downhill interface, Biomass-derived alcohols, ReS₂, MAPbBr₃, H₂ evolution

Tao Shan, Yanbo Li, Sunzai Ke, Bo Su, Lijuan Shen, Sibo Wang, Xuhui Yang, Min-Quan Yang. An embedded ReS₂@MAPbBr₃ heterostructure with downhill interfacial charge transfer for photocatalytic upgrading of biomass-derived alcohols to aldehydes and H₂[J]. J. Mater. Sci. Technol., 2024, 179: 155-165.

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An embedded ReS₂@MAPbBr₃ heterostructure with downhill interfacial charge transfer for photocatalytic upgrading of biomass-derived alcohols to aldehydes and H₂

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