Two-dimensional perovskite Pb2Nb3O10 photodetectors

doi:10.1016/j.jmst.2023.05.011

Abstract

Abstract: For the first time, we report high-performance two-dimensional (2D) perovskite Pb₂Nb₃O₁₀ photodetectors (PNO PDs). The few-layer PNO nanosheets are obtained successfully through a simple calcination and liquid exfoliation method. The individual PNO nanosheet devices with various structures (Au-PNO-Au, Au-PNO-Ti, Ti-PNO-Ti) are fabricated and investigated. The Au-PNO-Ti device exhibits a high rectification factor (∼10²) owing to a large Schottky barrier difference between the PNO nanosheet and two asymmetric electrodes. Notably, the Au-PNO-Ti device shows excellent self-powered performance, including high responsivity (2.8 A/W), high detectivity (1.1 × 10¹² Jones), and fast speed (0.2/1.2 ms) at 350 nm light illumination. This work not only suggests the performance of the PNO nanosheet PDs but also sheds light on the development of high-stability and high-performance devices based on 2D perovskite niobate in the future.

Key words: Pb₂Nb₃O₁₀, Photodetectors, Self-powered, Two-dimensional, Perovskite

Yong Zhang, Jian Yao, Zhen Zhang, Rong Zhang, Li Li, Yu Teng, Zongjie Shen, Lixing Kang, Limin Wu, Xiaosheng Fang. Two-dimensional perovskite Pb₂Nb₃O₁₀ photodetectors[J]. J. Mater. Sci. Technol., 2023, 164: 95-101.

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Two-dimensional perovskite Pb₂Nb₃O₁₀ photodetectors

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