Tunable and improved microwave absorption of flower-like core@shell MFe2O4@MoS2 (M = Mn, Ni and Zn) nanocomposites by defect and interface engineering

doi:10.1016/j.jmst.2022.08.022

J. Mater. Sci. Technol. ›› 2023, Vol. 139: 137-146.DOI: 10.1016/j.jmst.2022.08.022

• Research Article • Previous Articles Next Articles

Tunable and improved microwave absorption of flower-like core@shell MFe₂O₄@MoS₂ (M = Mn, Ni and Zn) nanocomposites by defect and interface engineering

Junxiong Xiao^a, Xiaosi Qi^a,b,*, Xiu Gong^a,*, Qiong Peng^a, Yanli Chen^a, Ren Xie^a, Wei Zhong^b,*

^aCollege of Physics, Guizhou Province Key Laboratory for Photoelectrics Technology and Application, Guizhou University, Guiyang 550025, China;
^bNational Laboratory of Solid State Microstructures and Jiangsu Provincial Laboratory for NanoTechnology, Nanjing University, Nanjing 210093, China

Received:2022-06-22 Revised:2022-07-22 Accepted:2022-08-11 Published:2023-03-10 Online:2023-03-06
Contact: *College of Physics, Guizhou Province Key Laboratory for Photoelectrics Technology and Application, Guizhou University, Guiyang City 550025, China. E-mail addresses: xsqi@gzu.edu.cn (X. Qi), xgong@gzu.edu.cn (X. Gong), wzhong@nju.edu.cn (W. Zhong) .

Abstract

Abstract: Previous results revealed that the defect and/or interface had a great impact on the electromagnetic parameters of materials. In order to understand the main physical mechanisms and effectively utilize these strategies, in this study, MFe₂O₄ and flower-like core@shell MFe₂O₄@MoS₂ (M = Mn, Ni, and Zn) samples with different categories were elaborately designed and selectively produced in large scale through a simple two-step hydrothermal reaction. We conducted the systematical investigation on their microstructures, electromagnetic parameters and microwave absorption performances (MAPs). The obtained results revealed that the large radius of M²⁺ cation could effectively boost the concentration of oxygen vacancy in the MFe₂O₄ and MFe₂O₄@MoS₂ samples, which resulted in the improvement of dielectric loss capabilities and MAPs. Furthermore, the introduction of MoS₂ nanosheets greatly improved the interfacial effect and enhanced the polarization loss capabilities, which also boosted the MAPs. By taking full advantage of the defect and interface, the designed MFe₂O₄@MoS₂ samples displayed tunable and excellent comprehensive MAPs including strong absorption capability, wide absorption bandwidth and thin matching thicknesses. Therefore, the clear understanding of defect and interface engineering made these strategies well elaborately designed and applicable to improving MAPs.

Key words: Core@shell structure, MFe₂O₄@MoS₂ (M=Mn, Ni and Zn), Defect and interface engineering, Improved microwave absorption properties

Junxiong Xiao, Xiaosi Qi, Xiu Gong, Qiong Peng, Yanli Chen, Ren Xie, Wei Zhong. Tunable and improved microwave absorption of flower-like core@shell MFe₂O₄@MoS₂ (M = Mn, Ni and Zn) nanocomposites by defect and interface engineering[J]. J. Mater. Sci. Technol., 2023, 139: 137-146.

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Tunable and improved microwave absorption of flower-like core@shell MFe₂O₄@MoS₂ (M = Mn, Ni and Zn) nanocomposites by defect and interface engineering

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