J. Mater. Sci. Technol. ›› 2023, Vol. 134: 189-196.DOI: 10.1016/j.jmst.2022.06.035
• Research Article • Previous Articles Next Articles
Zhe Hua,1, Hanxu Lua,1, Wenjie Zhoua, Jinxin Weia, Hanqing Daib, Hong Liua, Zhiyong Xiongb, Fengxian Xiea,c, Wanlu Zhanga,*(
), Ruiqian Guoa,b,c,d,*()
Received:2022-05-20
Revised:2022-06-11
Accepted:2022-06-15
Published:2023-01-20
Online:2023-01-10
Contact:
Wanlu Zhang,Ruiqian Guo
About author:rqguo@fudan.edu.cn (R. Guo).Zhe Hu, Hanxu Lu, Wenjie Zhou, Jinxin Wei, Hanqing Dai, Hong Liu, Zhiyong Xiong, Fengxian Xie, Wanlu Zhang, Ruiqian Guo. Aqueous synthesis of 79% efficient AgInGaS/ZnS quantum dots for extremely high color rendering white light-emitting diodes[J]. J. Mater. Sci. Technol., 2023, 134: 189-196.
Scheme 1. Schematic illustration for the QDs-PAAm/PVA fluorescent hydrogel films and their application in WLED.
Fig. 1. TEM and HRTEM images and histograms of the size distribution (inset) of (a, b) AIGS and (c, d) AIGS/ZnS QDs.
Fig. 2. Comparison of (a) XRD patterns, (b) XPS spectra, and (c) high-resolution XPS spectra of AIGS and AIGS/ZnS QDs.
Fig. 3. (a) UV-vis absorption spectra and the PL spectra (λex = 500 nm) with several batches of Zn-stock injection, (b) peak positions and PL QY of different batches of Zn-stock injection, and (c) PL decay curves and digital photographs under UV-light irradiation (inset) of AIGS and AIGS/ZnS QDs.
| Sample | τ1 (ns) | A1 (%) | τ2 (ns) | A2 (%) | τav (ns) |
|---|---|---|---|---|---|
| AIGS | 99.23 | 33.11 | 532.25 | 66.89 | 495.66 |
| AIGS/ZnS | 207.32 | 36.40 | 583.52 | 63.60 | 519.95 |
Table 1. Fitted parameters for PL decay curves of AIGS and AIGS/ZnS QDs.
| Sample | τ1 (ns) | A1 (%) | τ2 (ns) | A2 (%) | τav (ns) |
|---|---|---|---|---|---|
| AIGS | 99.23 | 33.11 | 532.25 | 66.89 | 495.66 |
| AIGS/ZnS | 207.32 | 36.40 | 583.52 | 63.60 | 519.95 |
Fig. 4. (a) UV-vis absorption spectra and the PL spectra (λex = 500 nm) of AIGS/ZnS QDs under different refluxing time. PL spectra (λex = 500 nm) of AIGS/ZnS QDs with different (b) refluxing temperatures, (c) pH values, and (d) GSH dosages.
Fig. 5. (a) UV-vis absorption spectra, normalized PL spectra (λex = 500 nm) and the corresponding digital photographs under UV-light irradiation (inset) of AIGS/ZnS QDs synthesized at different molar ratios of Ag/Ga. (b) Schematic diagram of the bandgap broadened by Ag proportion decrease.
Fig. 6. (a) PL spectra and (b) the corresponding digital photographs of green and red QDs-PAAm/PVA films under UV-light irradiation. (c) Electroluminescent spectrum and (d) CIE color coordinate of the WLED based on both green and red QDs-PAAm/PVA hydrogel films at a drive current of 100 mA.
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