J. Mater. Sci. Technol. ›› 2026, Vol. 265: 76-84.DOI: 10.1016/j.jmst.2025.10.077

• Research Article • Previous Articles     Next Articles

Heterodimensional co-decoration of carbon fibers with 2D MoS2 nanosheets and 0D Ag nanoparticles toward synergistically enhanced interfacial performance and electromagnetic attenuation in PEEK composites

Jiaqi Zhoua,b, Anping Zhua,b, Xiumei Zhanga,b, Baoming Wanga,b, Mingzhe Zhouc, Bo Zhua,b,*, Kun Qiaob,d,*   

  1. aCarbon Fiber Engineering Research Center, School of Materials Science and Engineering, Shandong University, Jinan 250061, China;
    bShandong Key Laboratory of Carbon Fiber and Composite Materials Manufacture and Application, Weihai 264211, China;
    cCentre for Atomaterials and Nanomanufacturing, School of Science, RMIT University, Melbourne, VIC 3000, Australia;
    dSchool of Mechanical, Electrical & Information Engineering, Shandong University, Weihai 264209, China
  • Received:2025-09-15 Revised:2025-10-24 Accepted:2025-10-29 Published:2026-09-10 Online:2025-11-28
  • Contact: * E-mail addresses: zhubo@sdu.edu.cn (B. Zhu), qiaokun@sdu.edu.cn (K. Qiao).

Abstract: The roll-out of 5 G communication has intensified electromagnetic (EM) pollution that not only disturbs electronic devices but also raises health concerns. Here, we report a hierarchical “face-to-point” architecture in which 2D MoS2 nanosheets are vertically grown on carbon fibers (CFs) and 0D Ag nanoparticles (AgNPs) are selectively anchored in the inter-sheet gaps. The resulting heterodimensional co-decoration acts as a 2D-0D synergistic “nano-nail” that simultaneously reinforces the interface and provides broadband EM attenuation. Hot pressed CF reinforced polyether ether ketone (CF/PEEK) composites exhibit a 66.21 % increase in interlaminar shear strength (ILSS, 95.44 MPa) and a 58.21 % boost in electromagnetic interference shielding effectiveness (EMI SET, 32.29 dB). Additionally, the UCF-M14@AgNPs demonstrated outstanding performance in electromagnetic wave (EMW) absorption, with a minimum reflection loss (RLmin) reaching -67.11 dB and an effective absorption bandwidth (EAB) extending up to 4.00 GHz. This dual-scale interfacial engineering strategy delivers structural composites that merge superior mechanical integrity with lightweight EM protection capability, offering immediate potential for aerospace and next-generation electronics.

Key words: CF with 2D MoS2 nanosheets and 0D AgNPs, CF/PEEK composite, Interfacial performance, Electromagnetic attenuation