Micro-sized hexapod-like CuS/Cu9S5 hybrid with broadband electromagnetic wave absorption

doi:10.1016/j.jmst.2024.07.014

Abstract

Abstract: Reasonable manipulation of component and microstructure is considered as a potential route to realize high-performance microwave absorber. In this paper, micro-sized hexapod-like CuS/Cu₉S₅ composites were synthesized via a facile approach involving the solvothermal method and subsequent sulfuration treatment. The resultant CuS/Cu₉S₅ exhibited superb microwave absorbing capacity with a minimum reflection loss (RL_min) of -59.38 dB at 2.7 mm. The maximum effective absorption bandwidth (EAB_max) was 7.44 GHz (10.56-18 GHz) when the thickness was reduced to 2.3 mm. The outstanding microwave absorbing ability of CuS/Cu₉S₅ composites is mainly related to its unique hexapod shape and the formation of heterogeneous interfaces. The unique hexapod shape significantly promotes the multi-reflection of the incident electromagnetic wave (EMW) increasing the attenuation path of EMWs in the material. Heterogeneous interfaces between CuS/Cu₉S₅ enable powerful interface polarization, contributing to the attenuation of EMWs propagating in the medium. In addition, the EMW absorption performance of CuS/Cu₉S₅ composites is also inseparable from the conduction loss. This study provides a strong reference for the research of EMW absorbent materials based on transition metal sulfides.

Key words: Heterogeneous interface, Hexapod shape, Transition metal sulfide, Electromagnetic wave absorption

Mengjun Han, Di Lan, Zhiming Zhang, Yizhi Zhao, Jiaxiao Zou, Zhenguo Gao, Guanglei Wu, Zirui Jia. Micro-sized hexapod-like CuS/Cu₉S₅ hybrid with broadband electromagnetic wave absorption[J]. J. Mater. Sci. Technol., 2025, 214: 302-312.

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Micro-sized hexapod-like CuS/Cu₉S₅ hybrid with broadband electromagnetic wave absorption

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