J. Mater. Sci. Technol. ›› 2026, Vol. 252: 147-153.DOI: 10.1016/j.jmst.2025.07.019

• Research Article • Previous Articles     Next Articles

Crystallized conjugated polymers constructed photonic synaptic transistors for in-sensor reservoir computing

Zhiyuan Zhaoa,b,1, Lu Huangc,1, Zhixuan Liua, Xingji Liua, Chen Lianga, Yingchao Hua, Wangyu Wud, Yayi Chena, Wei Zhonga, Jianfeng Zhanga, Xuecui Zoua, Dengyun Leia, Yao Nia,*, Xin Qinb,*, Yuan Liua,*   

  1. aSchool of Integrated Circuits, Guangdong University of Technology, Guangzhou 510006, China;
    bKey Laboratory of Ecological Restoration of Regional Contaminated Environment, Ministry of Education, College of Environment, Shenyang University, Shenyang 110044, China;
    cSchool of Physics &Optoelectronic Engineering, Guangdong University of Technology, Guangzhou 510006, China;
    dSchool of Computer Science, University of Liverpool, Liverpool L69 3DR, UK
  • Received:2025-05-11 Revised:2025-07-12 Accepted:2025-07-16 Published:2026-05-01 Online:2026-05-06
  • Contact: * E-mail addresses: niyao@gdut.edu.cn (Y. Ni), qinxinivy@126.com (X. Qin),eeliuyuan@gdut.edu.cn (Y. Liu) .
  • About author:1These authors contributed equally to this work.

Abstract: Neuromorphic computing continues to advance, fueling the pursuit of enhanced information processing and learning capabilities. This study introduces a novel photonic synaptic transistor (PST) based on crystallized conjugated polymers. Engineered to efficiently respond to standard temporal signals and digital images, this PST mimics the human retina's in-sensor computing mechanism. Developed through low-temperature solvent engineering, the PST optimizes charge carrier mobility and light absorption by finely tuning the polymer's microstructure. In a groundbreaking application, this PST has been used for image classification and Morse code recognition within reservoir computing frameworks. The polymer's microstructure modulation notably enhances the device's short-term and long-term plasticity, synaptic weight update efficiency, and training and recognition accuracy. These advancements underscore the potential of crystallized conjugated polymer-based PSTs to revolutionize next-generation neuromorphic computing systems.

Key words: Photonic synaptic transistor, Crystallized conjugated polymers, Short-term plasticity, Long-term plasticity, Reservoir computing