Recent advances in one-dimensional alkali-metal hexatitanate photocatalysts for environmental remediation and solar fuel production

doi:10.1016/j.jmst.2024.02.071

Abstract

Abstract: The global energy crisis and environmental problems have become two unprecedented challenges. Semiconductor photocatalysis offers a promising strategy to solve them, while its practical application requires advanced photocatalytic materials. In recent years, one-dimensional (1D) alkali-metal hexatitanate (AHT) photocatalysts have attracted considerable attention in energy and environmental fields due to their high chemical stability, excellent photoactivity, unique ion-exchange, environment-friendly, and cost-effective properties. In this review, we firstly introduce the basic properties of AHT including crystal and electronic band structure, photoactivity, and structure-property-performance relationship. Secondly, the recent advances in synthesis and modification strategies of 1D AHT photocatalysts are summarized thoughtfully, followed by a comprehensive discussion on their various environmental and energy applications, including pollutant degradation, H₂ generation, and CO₂ reduction. Finally, the key challenges and prospects are also highlighted for the development of high-performance 1D AHT-based photocatalysts for practical applications. We hope that this review will shed some light on the rational design of 1D Ti-O-based nanomaterials for efficient environmental remediation and solar fuel production.

Key words: Alkali-metal hexatitanates, One-dimensional nanomaterials, Photocatalysis, Pollutant degradation, Solar fuels

Qiang Wang, Xiaofan Yang, Zhao Jing, Hong Liu, Pengyi Tang, Hongmin Zhu, Bing Li. Recent advances in one-dimensional alkali-metal hexatitanate photocatalysts for environmental remediation and solar fuel production[J]. J. Mater. Sci. Technol., 2024, 202: 201-239.

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