Multiphase synergistic immobilization of complex trialkyl phosphine oxide end-waste into an iron-containing aluminosilicate glass-ceramic

doi:10.1016/j.jmst.2023.10.040

Abstract

Abstract: The objective of this study was to address the challenges associated with complex TRPO waste, by utilizing a natural aluminosilicate material to produce glass-ceramic waste forms. When the simulated waste content was below 30 wt.%, glassy waste forms were successfully obtained. Ce and Fe played crucial roles in the formation of Si-O-Ce bonds and [FeO₄]-tetrahedra in the glass network, which effectively immobilized other waste elements. However, when the waste content exceeded 30 wt.%, the waste was incorporated into feldspar, iron-manganese crystals, fluorite ceramic, and glass. This combination of ceramic and glass matrices synergistically immobilized the waste, resulting in excellent mechanical performance and chemical durability. The leaching rates of LR_Ce and LR_Nd were remarkably low around ∼10^-6 to 10^-7 g m^-2 d^-1, after 42 d. Furthermore, the study also investigated the role of multi-valence elements, such as Ce, Fe, and Mn, in the formation of iron-containing aluminosilicate glass-ceramics. The findings offer a novel approach to effectively immobilize complex nuclear waste.

Key words: Environmental protection, Complex nuclear waste, Aluminosilicate, Fluorite, Performance

Pan Tan, Xiaoyan Shu, Lijing Huang, Sihong Luo, Jing Chen, Yuexiang Lu, Mingfen Wen, Faqin Dong, Du Liu, Xiaoan Li, Xirui Lu. Multiphase synergistic immobilization of complex trialkyl phosphine oxide end-waste into an iron-containing aluminosilicate glass-ceramic[J]. J. Mater. Sci. Technol., 2024, 185: 83-97.

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