Dual strategy of A-site ion substitution and self-assembled MoS2 wrapping to boost permittivity for reinforced microwave absorption performance

doi:10.1016/j.jmst.2023.08.060

Abstract

Abstract: With the rapid development of electronic technology, how to effectively eliminate electromagnetic pollution has become a serious problem. Perovskite oxides have shown great potential in the field of electromagnetic wave absorption due to their unique structure and excellent physicochemical properties. Herein, by rationally manipulating the A-site ion substitution strategy, the theoretically directed doping of Sr ions into La ionic sites was utilized and the layered MoS₂ was loaded by the hydrothermal process to modify its surface. Consequently, the introduced polarization phenomenon improved the dielectric performance of the perovskite oxides, achieving a collaborative dielectric/magnetic loss mechanism. Accordingly, the prepared La_0.7Sr_0.3FeO₃(LSFO)/MoS₂ as coating filler in the epoxy resin coating system can obtain the minimum reflection loss of -67.09 dB at 1.9 mm and the maximum effective absorption bandwidth of 7.28 GHz at 2.3 mm. More importantly, it also exhibits excellent absorption performance for multi-band electromagnetic waves, covering a wide range of specified frequency bands. It provides inspiration for exploring novel perovskite oxide-based electromagnetic wave absorbing coatings and broadens the choice of ideal candidate materials for designing highly efficient, multi-band absorbers to cope with sophisticated electromagnetic environments.

Key words: Perovskite oxides, A-site ion substitution, Multi-band, Electromagnetic wave absorbing coating

Ailing Feng, Di Lan, Jinkun Liu, Guanglei Wu, Zirui Jia. Dual strategy of A-site ion substitution and self-assembled MoS₂ wrapping to boost permittivity for reinforced microwave absorption performance[J]. J. Mater. Sci. Technol., 2024, 180: 1-11.

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Dual strategy of A-site ion substitution and self-assembled MoS₂ wrapping to boost permittivity for reinforced microwave absorption performance

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