A hierarchical Bi-MOF-derived BiOBr/Mn0.2Cd0.8S S-scheme for visible-light-driven photocatalytic CO2 reduction

doi:10.1016/j.jmst.2023.03.003

Abstract

Abstract: S-scheme heterojunctions have promising applications in photocatalytic CO₂ reduction due to their unique structure and interfacial interactions, but improving their carrier separation efficiency and CO₂ adsorption capacity remains a challenge. In this work, highly dispersed MOF-BiOBr/Mn_0.2Cd_0.8S (MOF-BiOBr/MCS) S-scheme heterojunctions with high photocatalytic CO₂ reduction performance were constructed. The intimate contact between the MCS nano-spheres and the nanosheet-assembled MOF-BiOBr rods, driven by the internal electric field, accelerates the charge transfer along the S-scheme pathway. Moreover, the high specific surface area of MOFs is preserved to provide abundant active sites for reaction/adsorption. The formation of MOF-BiOBr/MCS S-scheme heterojunction is confirmed by theoretical calculations. The optimum MOF-BiOBr/MCS shows excellent activity in CO₂ reduction, affording a high CO evolution rate of 60.59 µmol h^-1 g^-1. The present work can inspire the exploration for the construction of effective heterostructure photocatalysts for photoreduction CO₂.

Key words: Mn_0.2Cd_0.8S, Bi-MOF, CO₂ reduction, S-scheme heterojunction

Jiahui Hua, Zhongliao Wang, Jinfeng Zhang, Kai Dai, Chunfeng Shao, Ke Fan. A hierarchical Bi-MOF-derived BiOBr/Mn_0.2Cd_0.8S S-scheme for visible-light-driven photocatalytic CO₂ reduction[J]. J. Mater. Sci. Technol., 2023, 156: 64-71.

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A hierarchical Bi-MOF-derived BiOBr/Mn_0.2Cd_0.8S S-scheme for visible-light-driven photocatalytic CO₂ reduction

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