J. Mater. Sci. Technol. ›› 2020, Vol. 46: 88-97.DOI: 10.1016/j.jmst.2019.12.012
• Research Article • Previous Articles Next Articles
Bowen Zhaoa,b, Zhengwang Zhua,*(), Xin Dong Qinc, Zhengkun Lia, Haifeng Zhanga
Received:
2019-11-03
Revised:
2019-12-22
Accepted:
2019-12-30
Published:
2020-06-01
Online:
2020-06-19
Contact:
Zhengwang Zhu
Bowen Zhao, Zhengwang Zhu, Xin Dong Qin, Zhengkun Li, Haifeng Zhang. Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation[J]. J. Mater. Sci. Technol., 2020, 46: 88-97.
Fig. 1. (a) XRD patterns and (b) DSC curves of melt-spun CuZr-based metallic glass ribbons, (c) HRTEM image and (d) SAED pattern of the melt-spun Cu47.5Zr46Al6.5 metallic glass ribbons.
Fig. 2. (a) Typical UV-vis spectra of AO Ⅱ aqueous solution degraded by Cu47.5Zr46Al6.5 metallic glassy ribbons, (b) the normalized concentration of AO Ⅱ aqueous solution at 484 nm treated by samples of different Cu contents as a function of reaction time, (c) the normalized concentration of AO Ⅱ aqueous solution at 484 nm treated by samples of different Al contents as a function of reaction time, (d) the comparison of degradation efficiency and degradation rate for six different composition ribbons (AO Ⅱ: 100 mg/L, surface area of ribbons: 1000 cm2/L, temperature: 313 K, pH = 2).
Fig. 3. Effect of (a) surface area of ribbons, (b) temperature and (c) pH on the normalized concentration of AO Ⅱ aqueous solution using Cu47.5Zr46Al6.5 metallic glassy ribbons, (d) the degradation efficiency of AO Ⅱ aqueous solution with Cu47.5Zr46Al6.5 metallic glassy ribbons at the different cycles (if not mentioned, AO Ⅱ: 100 mg/L, surface area of ribbons: 1000 cm2/L, temperature: 313 K, pH = 2).
Fig. 4. Effect of (a) additive types and (b) c(H+) and c(Cl-) on the normalized concentration of AO Ⅱ aqueous solution using Cu47.5Zr46Al6.5 metallic glassy ribbons, surface morphology of the Cu47.5Zr46Al6.5 metallic glassy ribbons after degradation with the different additive types of (c) NaCl solution, (d) H2SO4 solution, (e) NaCl and H2SO4 solution, (f) HCl solution (if not mentioned, AO Ⅱ: 100 mg/L, surface area of ribbons: 1000 cm2/L, temperature: 313 K, pH = 2).
Fig. 6. (a) SEM image of EDS analysis (inset) of melt-spun Cu47.5Zr46Al6.5 metallic glassy ribbons, (b) SEM image of EDS analysis (inset) of first reacted Cu47.5Zr46Al6.5 metallic glassy ribbons, (c) SEM image of third reacted Cu47.5Zr46Al6.5 metallic glassy ribbons, (d) SEM image and (f) low magnification SEM image of eighth reacted Cu47.5Zr46Al6.5 metallic glassy ribbons, (e) SEM image, (g) low magnification SEM image and (h) mapping results of tenth reacted Cu47.5Zr46Al6.5 metallic glassy ribbons.
Fig. 7. XPS spectrum of (a) the full range spectrum, (b) Cu 2p, (c) Zr 3d and (d) Al 1 s in binding energy regions for the as-spun and reacted Cu47.5Zr46Al6.5 metallic glassy ribbons.
[1] | Q.Q. Wang, M.X. Chen, P.H. Lin, Z.Q. Cui, C.L. Chu, B.L. Shen, J. Mater. Chem. A 6 (2018) 10686-10699. |
[2] | Y.X. Qin, L.Z. Zhang, T.C. An, ACS Appl. Mater. Interfaces 9 (2017) 17115-17124. |
[3] | U.G. Akpan, B.H. Hameed, J. Hazard. Mater. 170(2009) 520-529. |
[4] |
H.D. Chen, J.K. Xu, J.Q. Wei, P.F. Wang, Y.B. Han, J.C. Xu, B. Hong, H.X. Jin, D.F. Jin, X.L. Peng, J. Li, Y.T. Yang, H.L. Ge, X.Q. Wang, J. Phys. Chem. Solids 132 (2019) 138-144.
DOI URL |
[5] |
R. Bhavani, A. Sivasamy, Ecotoxicol. Environ. Saf. 134(2016) 403-411.
DOI URL |
[6] |
P. Borker, A.V. Salker, Mater. Sci. Eng. B. 133(2006) 55-60.
DOI URL |
[7] |
S. Das, S. Garrison, S. Mukherjee, Adv. Eng. Mater. 18(2016) 214-218.
DOI URL |
[8] |
S.Y. Yang, X. Yang, X.T. Shao, R. Niu, L.L. Wang, J. Hazard. Mater. 186(2011) 659-666.
DOI URL |
[9] | P.K. Malik, J. Hazard. Mater. 113(2004) 81-88. |
[10] |
M.B. Ahmed, J.L. Zhou, H.H. Ngo, W.S. Guo, N.S. Thomaidis, J. Xu, J. Hazard. Mater. 323(2017) 274-298.
DOI URL |
[11] |
Y. Tang, Y. Shao, N. Chen, X. Liu, S.Q. Chen, K.F. Yao, RSC Adv. 5(2015) 34032-34039.
DOI URL |
[12] |
H. Ma, Y.P. Huang, M.W. Shen, D.M. Hu, H. Yang, M.F. Zhu, S.P. Yang, X.Y. Shi, RSC Adv. 3(2013) 6455-6465.
DOI URL |
[13] |
A. J.Salter-Blanc, P.G. Tratnyek, Environ. Sci. Technol. 45(2011) 4073-4079.
DOI URL |
[14] |
C. Cai, Z.Y. Zhang, J. Liu, N. Shan, H. Zhang, D.D. Dionysiou, Appl. Catal. B: Environ. 182(2016) 456-468.
DOI URL |
[15] | J.M. Chacón, M.T. Leal, M. Sánchez, Er.R. Bandala, Dyes Pigm. 69(2006) 144-150. |
[16] |
L.C. Zhang, S.X. Liang, Chem. Asian J. 13(2018) 3575-3592.
DOI URL |
[17] |
D.G. Bassyouni, H.A. Hamad, E.-S.Z. El-Ashtoukhy, N.K. Amin, M.M. Abd El-Latif, J. Hazard. Mater. 335(2017) 178-187.
DOI URL |
[18] |
X.D. Qin, Z.K. Li, Z.W. Zhu, H.M. Fu, H. Li, A.M. Wang, H.W. Zhang, H.F. Zhang, J. Mater. Sci. Technol. 34(2018) 2290-2296.
DOI URL |
[19] |
H.Y. Min, X.Q. Ran, J.W. Fan, Y. Sun, J.P. Yang, W. Teng, W.X. Zhang, G.M. Li, D.Y. Zhao, J. Mater. Chem. A. 3(2015) 7399-7405.
DOI URL |
[20] | R. Li, X.J. Liu, H. Wang, Y. Wu, K.C. Chan, Z.P. Lu, Mater. Design. 155(2018) 346-351. |
[21] | S.X. Liang, Z. Jia, Y.J. Liu, W.C. Zhang, W.M. Wang, J. Lu, L.C. Zhang, Adv. Mater. 30(2018), 180276. |
[22] |
Z. Jia, X.G. Duan, P. Qin, W.C. Zhang, W.M. Wang, C. Yang, H.Q. Sun, S.B. Wang, L.C. Zhang, Adv. Funct. Mater. 27(2017), 1702258.
DOI URL |
[23] | J.C. Wang, S.X. Liang, Z. Jia, W.C. Zhang, W.M. Wang, Y.J. Liu, J. Lu, L.C. Zhang, J. Alloys. Compd. 728(2017) 525-533. |
[24] |
L. Xu, W. Wei, H.X. Li, H. Li, ACS Catal. 4(2014) 251-258.
DOI URL |
[25] |
F. Hu, S.L. Zhu, S.M. Chen, Y. Li, L. Ma, T.P. Wu, Y. Zhang, C.M. Wang, C.C. Liu, X.J. Yang, L. Song, X.W. Yang, Y.J. Xiong, Adv. Mater. 29(2017), 1606570.
DOI URL |
[26] |
W.H. Wang, Adv. Mater. 21(2009) 4524-4544.
DOI URL |
[27] |
J.Q. Wang, Y.H. Liu, M.W. Chen, D.V.Louzguine-Luzgin, A.Inoue, J.H. Perepezko, Sci. Rep. 2(2012) 418.
DOI URL |
[28] |
M. Ramya, M. Karthika, R. Selvakumar, Baldev Raj, K.R. Ravi, J. Alloys Compd. 696(2017) 185-192.
DOI URL |
[29] |
Y.F. Zhao, J.J. Si, J.G. Song, Q. Yang, X.D. Hui, Mater. Sci. Eng. B. 181(2014) 46-55.
DOI URL |
[30] |
X.K. Luo, R. Li, J.Z. Zong, Y. Zhang, H.F. Li, T. Zhang, Appl. Surf. Sci. 305(2014) 314-320.
DOI URL |
[31] |
P.P. Wang, J.Q. Wang, H. Li, H. Yang, J.T. Huo, J.G. Wang, C.T. Chang, X.M. Wang, R.W. Li, G. Wang, J. Alloys. Compd. 701(2017) 759-767.
DOI URL |
[32] | W. Ben Mbarek, M. Azabou, E. Pineda, N. Fiol, L. Escoda, J.J. Sunol, M. Khitouni, RSC Adv. 7(2017) 12620-12628. |
[33] |
X.D. Qin, Z.W. Zhu, G. Liu, H.M. Fu, H.W. Zhang, A.M. Wang, H. Li, H.F. Zhang, Sci. Rep. 5(2015) 18226.
DOI URL |
[34] | C.Q. Zhang, Q.L. Sun, K.G. Liu, J. Alloys. Compd. 741(2018) 1040-1047. |
[35] |
Z. Jia, J.C. Wang, S.X. Liang, W.C. Zhang, W.M. Wang, L.C. Zhang, J. Alloys. Compd. 728(2017) 525-533.
DOI URL |
[36] |
C.Q. Zhang, Z.W. Zhu, H.F. Zhang, Z.Q. Hu, J. Non-Cryst. Solids 358 (2012) 61-64.
DOI URL |
[37] | J.Q. Wang, Y.H. Liu, M.W. Chen, G.Q. Xie, D.V.Louzuine-Luzgin, A.Inoue, J.H. Perepezko, Adv. Funct. Mater. 22(2012) 2567-2570. |
[38] | X.L. Li, Y.Y. Wu, S.T. Yang, X.J. Cha, P.C. Shao, L. Wang, J. Non-Cryst. Solids 503-504(2019) 284-287. |
[39] |
Z. Jia, W.C. Zhang, W.M. Wang, D. Habibi, L.C. Zhang, Appl. Catal. B: Environ. 192(2016) 46-56.
DOI URL |
[40] |
X.D. Qin, Z.K. Li, Z.W. Zhu, H.M. Fu, H. Li, A.M. Wang, H.W. Zhang, H.F. Zhang, J. Mater. Sci. Technol. 33(2017) 1147-1152.
DOI URL |
[41] | Z. Deng, X.H. Zhang, K.C. Chan, L. Liu, T. Li, Chemosphere 174 (2017) 76-81. |
[42] | W.M. Yang, Q.Q. Wang, W.Y. Li, L. Xue, H.S. Liu, J. Zhou, Mater. Design. 161(2019) 136-146. |
[43] |
Z. Jia, J. Kang, W.C. Zhang, W.M. Wang, C. Yang, H. Sun, D. Habibi, L.C. Zhang, Appl. Catal. B: Environ. 204(2017) 537-547.
DOI URL |
[44] |
B. Zhang, J. Wang, B. Wu, X.W. Guo, Y.J. Wang, D. Chen, Y.C. Zhang, K. Du, E.E. Oguzie, X.L. Ma, Nat. Commun. 9(2018) 2559.
DOI URL |
[45] | M.P. Ryan, D.E. Williams, R.J. Chater, B.M. Hutton, D.S. Mcphail, Nature 415 (2002) 770-774. |
[46] | F. Guan, J.Z. Duan, X.F. Zhai, N. Wang, J. Zhang, D.Z. Lu, B.R. Hou, J. Mater. Sci. Technol. 36(2020) 55-64. |
[47] |
C. Yang, C. Zhang, L. Liu, J. Mater. Chem. A. 6(2018) 20992-21002.
DOI URL |
[48] |
S.S. Wang, L. Liu, J. Hazard. Mater. 340(2017) 445-453.
DOI URL |
[49] |
N. Wang, Y. Pan, S.K. Wu, E.M. Zhang, W.J. Dai, RSC Adv. 7(2017) 43255-43265.
DOI URL |
[50] |
M. AboliGhasemabadi, W.B. Mbarek, O. Casabella, H. Roca-Bisbe, E. Pineda, L. Escoda, J.J. Suñold, J. Alloys. Compd. 741(2018) 240-245.
DOI URL |
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