Flexible thermoregulatory microcapsule/polyurethane-MXene composite films with multiple thermal management functionalities and excellent EMI shielding performance

doi:10.1016/j.jmst.2023.05.013

材料科学与技术 ›› 2023, Vol. 165 ›› Issue (0): 27-38.DOI: 10.1016/j.jmst.2023.05.013

收稿日期:2023-04-14 修回日期:2023-05-02 接受日期:2023-05-03 出版日期:2023-12-01 发布日期:2023-06-10

Flexible thermoregulatory microcapsule/polyurethane-MXene composite films with multiple thermal management functionalities and excellent EMI shielding performance

Danyuan Huang^a, Ying Chen^b, Li Zhang^a,b, Xinxin Sheng^a,b,*

^aDepartment of Polymeric Materials and Engineering, School of Materials and Energy, Guangdong University of Technology, Guangzhou, 510006, China;
^bGuangdong Provincial Key Laboratory of Functional Soft Condensed Matter, Guangdong University of Technology, Guangzhou, 510006, China

Received:2023-04-14 Revised:2023-05-02 Accepted:2023-05-03 Online:2023-12-01 Published:2023-06-10
Contact: *E-mail address: . xinxin.sheng@gdut.edu.cn (X. Sheng)

摘要/Abstract

Abstract: The development of miniaturized, flexible, and portable electronic devices has led to an increasing demand for multifunctional flexible films that can provide temperature regulation, electromagnetic interference (EMI) shielding, and thermal management. In this study, a novel hierarchical multifunctional flexible composite film is presented. The first step involves the synthesis of phase change microcapsule (PCMC) latex through in-situ polymerization. Next, PCMC and waterborne polyurethane (WPU) latex were mixed and dried using a binary colloidal approach to produce a flexible composite phase change film (WPU/PCMC) with complete anti-leakage and satisfying melting enthalpy (147.86 J g^-1). To enhance the EMI performance and mechanical strength, a thin layer of antioxidant MXene@poly tannin acid (PTA) was directly sprayed onto the surface of WPU/PCMC, resulting in the WPU/PCMC/MXene@PTA film (WPM). Consequently, the WPM displays exceptional thermal management performance for multiple drives and outstanding EMI performance (56.86 dB), making it an ideal candidate for future multifunctional products.

Key words: Flexibility, Microcapsules, Composite film, Thermal management, EMI shielding

. [J]. 材料科学与技术, 2023, 165(0): 27-38.

Danyuan Huang, Ying Chen, Li Zhang, Xinxin Sheng. Flexible thermoregulatory microcapsule/polyurethane-MXene composite films with multiple thermal management functionalities and excellent EMI shielding performance[J]. J. Mater. Sci. Technol., 2023, 165(0): 27-38.

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Flexible thermoregulatory microcapsule/polyurethane-MXene composite films with multiple thermal management functionalities and excellent EMI shielding performance

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