材料科学与技术 ›› 2022, Vol. 120 ›› Issue (0): 65-77.DOI: 10.1016/j.jmst.2021.10.055
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收稿日期:2021-07-30修回日期:2021-10-10接受日期:2021-10-20出版日期:2022-09-01发布日期:2022-02-24
Formation process and oxidation behavior of MCrAlY + AlSiY composite coatings on a Ni-based superalloy
S.M. Lia,b, L.B. Fua,b, W.L. Zhanga,b, W. Lib,*(
), J. Sunc, T.G. Wangd, S.M. Jiangb,*(), J. Gongb, C. Sunb,*()
- aSchool of Materials Science and Engineering, University of Science and Technology of China, Shenyang 110016, China
bShi-changxu Innovation Center for Advanced Materials, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, China
CAdvanced Research Institute for Multidisciplinary Science, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China
DTianjin Key Laboratory of High Speed Cutting and Precision Machining, Tianjin University of Technology and Education, Tianjin 300222, China
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Received:2021-07-30Revised:2021-10-10Accepted:2021-10-20Online:2022-09-01Published:2022-02-24 -
Contact:W. Li,S.M. Jiang,C. Sun -
About author:* E-mail addresses: wli@imr.ac.cn (W. Li),
引用本文
. [J]. 材料科学与技术, 2022, 120(0): 65-77.
S.M. Li, L.B. Fu, W.L. Zhang, W. Li, J. Sun, T.G. Wang, S.M. Jiang, J. Gong, C. Sun. Formation process and oxidation behavior of MCrAlY + AlSiY composite coatings on a Ni-based superalloy[J]. J. Mater. Sci. Technol., 2022, 120(0): 65-77.
Fig. 1. Schematic drawing of detailed preparation processes for three coatings.
| Empty Cell | NiCrAlYSi target | AlSiY target |
|---|---|---|
| Arc voltage (V) | 19-21 | 19-21 |
| Arc current (A) | 80-90 | 80-90 |
| Bias voltage (-V) | 160 | 120 |
| Bias duty cycle (%) | 30 | 30 |
| Target-substrate distance(mm) | 120 | 120 |
| Air pressure (Pa) | 0.22-0.24 | 0.3 |
| Temperature (°C) | 300-400 | 300-400 |
Table 1. Deposition parameters of arc ion plating.
| Empty Cell | NiCrAlYSi target | AlSiY target |
|---|---|---|
| Arc voltage (V) | 19-21 | 19-21 |
| Arc current (A) | 80-90 | 80-90 |
| Bias voltage (-V) | 160 | 120 |
| Bias duty cycle (%) | 30 | 30 |
| Target-substrate distance(mm) | 120 | 120 |
| Air pressure (Pa) | 0.22-0.24 | 0.3 |
| Temperature (°C) | 300-400 | 300-400 |
Fig. 2. Cross-sectional morphologies of C1 during annealing process, (a) as-deposited, (b) heated to 700 °C, (c) heated to 900 °C, (d) heated to 1000 °C and held for 30 min, (e) at the ending of annealing, (f-h) bright-field images of precipitates in the outermost layer of annealed C1.
| Location | Average composition | ||||||
|---|---|---|---|---|---|---|---|
| Al | Si | Cr | Co | Ni | W | Ti | |
| zone 1 in the C1 | 45.4 | 1 | 5.2 | 5.4 | 38.1 | 3.4 | 1.5 |
| zone 2 in the C1 | 40 | 1 | 6.4 | 6.4 | 39.1 | 5.4 | 1.7 |
| zone 3 in the C1 | 34.1 | 2.1 | 6.4 | 7.3 | 40.4 | 8.6 | 2.1 |
| zone 4 in the C1 | 24.1 | 1.3 | 6.4 | 8.4 | 50.7 | 8.1 | 1 |
| zone 5 in the C1 | 24.1 | 1.7 | 7.8 | 8 | 49.3 | 7.6 | 1.4 |
| zone 6 in the C1 | 23.4 | — | 4.5 | 9.3 | 60 | 2.8 | — |
| zone 1 in the C2 | 43.5 | 2.1 | 14 | — | 40.4 | — | — |
| zone 2 in the C2 | 33.3 | 3.4 | 17 | — | 46.3 | — | — |
| zone 3 in the C2 | 39.6 | 0.6 | 13.4 | — | 46.4 | — | — |
| zone 4 in the C2 | 35.4 | 0.4 | 15.7 | — | 48.5 | — | — |
| zone 7 in the C2 | 24.8 | 3 | 16.4 | — | 55.8 | — | — |
| zone 8 in the C2 | 25.4 | 0.3 | 11.8 | 0.7 | 61.8 | — | — |
| zone 10 in the C2 | 23.7 | 3 | 16.3 | 0.7 | 56.3 | — | — |
| zone 11 in the C2 | 15 | — | 29.9 | 4.6 | 48.3 | 2.3 | — |
| zone 5 in the C3 | 21.8 | 1.8 | 14 | 0.4 | 62 | — | — |
| zone 6 in the C3 | 13.6 | — | 32.1 | 2.6 | 49.6 | 2.1 | — |
Table 2. The average compositions of coatings (wt.%).
| Location | Average composition | ||||||
|---|---|---|---|---|---|---|---|
| Al | Si | Cr | Co | Ni | W | Ti | |
| zone 1 in the C1 | 45.4 | 1 | 5.2 | 5.4 | 38.1 | 3.4 | 1.5 |
| zone 2 in the C1 | 40 | 1 | 6.4 | 6.4 | 39.1 | 5.4 | 1.7 |
| zone 3 in the C1 | 34.1 | 2.1 | 6.4 | 7.3 | 40.4 | 8.6 | 2.1 |
| zone 4 in the C1 | 24.1 | 1.3 | 6.4 | 8.4 | 50.7 | 8.1 | 1 |
| zone 5 in the C1 | 24.1 | 1.7 | 7.8 | 8 | 49.3 | 7.6 | 1.4 |
| zone 6 in the C1 | 23.4 | — | 4.5 | 9.3 | 60 | 2.8 | — |
| zone 1 in the C2 | 43.5 | 2.1 | 14 | — | 40.4 | — | — |
| zone 2 in the C2 | 33.3 | 3.4 | 17 | — | 46.3 | — | — |
| zone 3 in the C2 | 39.6 | 0.6 | 13.4 | — | 46.4 | — | — |
| zone 4 in the C2 | 35.4 | 0.4 | 15.7 | — | 48.5 | — | — |
| zone 7 in the C2 | 24.8 | 3 | 16.4 | — | 55.8 | — | — |
| zone 8 in the C2 | 25.4 | 0.3 | 11.8 | 0.7 | 61.8 | — | — |
| zone 10 in the C2 | 23.7 | 3 | 16.3 | 0.7 | 56.3 | — | — |
| zone 11 in the C2 | 15 | — | 29.9 | 4.6 | 48.3 | 2.3 | — |
| zone 5 in the C3 | 21.8 | 1.8 | 14 | 0.4 | 62 | — | — |
| zone 6 in the C3 | 13.6 | — | 32.1 | 2.6 | 49.6 | 2.1 | — |
Fig. 3. XRD patterns for C1 during annealing process.
Fig. 4. Cross-sectional morphologies of C2 during annealing process, (a) as-deposited, (b) heated to 700 °C, (c) heated to 900 °C, (d) heated to 1000 °C and held for 30 min, (e) at the ending of annealing, (f, g) bright-field images of annealed C2.
Fig. 5. XRD patterns for C2 during annealing process.
Fig. 6. Cross-sectional morphologies of C3 during annealing process, (a) as-deposited, (b) heated to 700 °C, (c) heated to 900 °C, (d) heated to 1000 °C and held for 30 min, (e) at the ending of annealing.
Fig. 7. XRD patterns for C3 during annealing process.
Fig. 8. Isothermal oxidation kinetic curves for coatings at 1100 °C, (a) total mass change, (b) square of mass gain versus oxidation time of coating, which displayed the oxidation rate constant (kp).
Fig. 9. XRD patterns of coatings after 50 and 200 h isothermal oxidation at 1100 °C, (a) C1, (b) C2 and (c) C3.
Fig. 10. Cross-sectional images of coatings after isothermal oxidation at 1100 °C, (a, d) C1, (b, e) C2, (c, f) C3, (a-c) for 50 h, (d-f) for 300 h.
Fig. 11. Surface images of coatings after isothermal oxidation at 1100 °C, (a, d) C1, (b, e) C2, (c, f) C3, (a-c) for 50 h, (d-f) for 300 h.
Fig. 12. Raman spectrogram of Al2O3 scale formed on the coating.
Fig. 13. Schematic drawing of coatings formation in vacuum annealing process.
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